Aerosol-cloud interactions remain the largest uncertainty in climate projections. Ultrafine aerosol particles smaller than 50 nanometers (UAP) can be abundant in the troposphere but are conventionally considered too small to affect cloud formation. Observational evidence and numerical simulations of deep convective clouds (DCCs) over the Amazon show that DCCs forming in a low-aerosol environment can develop very large vapor supersaturation because fast droplet coalescence reduces integrated droplet surface area and subsequent condensation. UAP from pollution plumes that are ingested into such clouds can be activated to form additional cloud droplets on which excess supersaturation condenses and forms additional cloud water and latent heating, thus intensifying convective strength. This mechanism suggests a strong anthropogenic invigoration of DCCs in previously pristine regions of the world.

One of the least understood aspects in atmospheric chemistry is how urban emissions influence the formation of natural organic aerosols, which affect Earth’s energy budget. The Amazon rainforest, during its wet season, is one of the few remaining places on Earth where atmospheric chemistry transitions between preindustrial and urban-influenced conditions. Here, we integrate insights from several laboratory measurements and simulate the formation of secondary organic aerosols (SOA) in the Amazon using a high-resolution chemical transport model. Simulations show that emissions of nitrogen-oxides from Manaus, a city of ~2 million people, greatly enhance production of biogenic SOA by 60–200% on average with peak enhancements of 400%, through the increased oxidation of gas-phase organic carbon emitted by the forests. Simulated enhancements agree with aircraft measurements, and are much larger than those reported over other locations. The implication is that increasing anthropogenic emissions in the future might substantially enhance biogenic SOA in pristine locations like the Amazon.

This paper aims to identify the circulation associated with Easterly Wave Disturbances (EWDs) that propagate toward the Eastern Northeast Brazil (ENEB) and their impact on the rainfall over ENEB during 2006 and 2007 rainy seasons (April–July). The EWDs identification and trajectory are analyzed using an automatic tracking technique (TracKH). The EWDs circulation patterns and their main features were obtained using the composite technique. To evaluate the TracKH efficiency, a validation was done by comparing the EWDs number tracked against observed cases obtained from an observational analysis. The mean characteristics of EWDs are 5.5-day period, propagation speed of ~9.5 m·s−1, and a 4500 km wavelength. A synoptic analysis shows that between days −2 d and 0 d, the low level winds presented cyclonic relative vorticity and convergence anomalies both in 2006 and 2007. The EWDs signals are strongest at low levels. The EWDs propagation is associated with relative humidity and precipitation positive anomalies and OLR and omega negative anomalies. The EWDs tracks are seen over all ENEB and their lysis occurs between the ENEB and marginally inside the continent. The tracking captured 71% of EWDs in all periods, indicating that an objective analysis is a promising method for EWDs detection.

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A 21-yr climatology of Easterly Waves Disturbances (EWDs) over the Tropical South Atlantic (TSA) has been examined using data from the European Centers for Medium-Range Weather Forecasting (ECMWF) interim reanalysis (ERAI) and satellite data. This includes the frequency distribution of EWDs and their interannual variability. The largescale environment associated with EWDs has been investigated for the coastal region of Northeast Brazil (NEB) for the rainy (April-August) season using a composite analysis. EWDs were first identified in ERAI, resulting in 518 observed cases. These were found to show notable interannual variability with around 16-40 episodes each year and with an average lifetime of 4-6 days. Of the identified EWDs, 97% reached the coast of NEB, of which 64% were convective in nature and 14% moved across the NEB region and reached the Amazon. The annual occurrence of EWDs seems to be lower (higher) during El Niño (La Niña). The monthly occurrence of EWDs shows higher activity in the rainy season. EWDs originate in association with five types of system: cold fronts, convective clusters from the west coast of Africa, Intertropical Convergence Zone and Tropical Upper Tropospheric Cyclonic Vortices. The composite analysis indicates strong relative vorticity (RV) and divergence anomalies at low levels, as well as in the vertical profiles of relative humidity and vertical velocity (omega). The precipitation composites show that the EWDs propagate between the TSA and NEB and contribute at least 60% of the total rainfall over the east coast of NEB throughout the rainy season.