The interfacial Dzyaloshinskii–Moriya interaction (DMI) in ferromagnetic/non‐magnetic‐metal bilayers is essential to stabilize chiral spin textures for potential applications. Recent works reveal that the interlayer DMI is beneficial to designing 3D chiral spin textures that possess fundamental importance and the associated technological promises. Here, the interlayer DM constants are determined quantitatively in synthetic ferromagnetic/antiferromagnetic Pt/Co/Pt/Ru/Pt/Co/Ta structures. The results demonstrate that the interlayer DMI shows uniaxial anisotropic characteristics. The first‐principles calculations elucidate that the anisotropic interlayer DMI is induced by the in‐plane symmetry breaking along two high symmetric directions, which favors the magnetization of adjacent ferromagnetic layers canting in different directions. The anisotropic interlayer DMI is also confirmed by spin‐orbit torque driven asymmetric magnetization switching. Moreover, the interlayer DMI can be tuned by the Ru‐layer‐thickness and beneficial to designing 3D spin textures for future spintronic devices.

The spin-orbit torque via the spin Hall effect of heavy metals has shown promising prospect in driving the magnetization switching in spintronic devices due to the generated spin current from heavy metals. Recently, the 3d-light metals have been predicted the ability to generate orbital current and the associated orbital torques from the orbital Hall effect. However, few experiments have been carried out since it’s quite hard to directly detect the orbital current generated orbital torque. Here, we report an effective method to demonstrate the strong orbital torques in light metal Cr through a conversion process from orbital current to spin current by introducing the Pt interfacial layer in perpendicular magnetized symmetric Pt/Co/Pt structures. A quite large and monotonically growth of orbital torque efficiency in Pt/Co/Pt/Cr with the increase of the thickness of Cr layer is obtained with the largest effective orbital torque efficiency around 2.6 Oe/(MA·cm-2). The ability of orbital torque to drive the magnetization switching is also reported with the critical switching current density down to the order of 106 A·cm-2. Our findings prove the efficiency for switching the magnetization from light metal Cr layers through the orbital Hall effect.

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The spin–orbit torques originating from the spin Hall effect of heavy metals are of vital importance for applications in spintronics due to its low consumption of energy. Theoretical calculations have predicted that 3 d and 4 d light metals can produce a similar amount of torques to heavy metals via the strong orbital Hall effect (OHE). However, few experiments have been conducted since it is technically challenging to directly detect the orbital current from the OHE. Here, we report an effective approach to demonstrate the strong orbital torques in the light metal Cr with the aid of a conversion process from the orbital current to the spin current by introducing an Au interfacial layer in the Cr/ferromagnet structures. A rather large orbital torque efficiency and an increase with the increasing thickness of the Cr-layer are attained in the perpendicularly magnetized Cr/Au/Co/Ti multilayers. Moreover, an energy efficient magnetization switching and the domain wall motion in Cr/Au/Co/Ti multilayers induced by the OHE have also been observed. Our findings confirm the existence of the orbital Hall torques in Cr and provide an effective way to investigate the OHE.