We report all-optically controlled fourth- and sixth-order fluorescence processes with and without splitting, in a heteronuclear-like molecule system of Pr3+:YSO both in theory and experiment. We construct the asymptote among Pr3+ ions localized at different cation vacancies. By changing the frequency detuning and power of the controlling field, fluorescence signal can be controlled to switch from an enhanced peak to a suppressed dip, and vice versa. Such transition has a potential application to produce all-optical switches. The results can be well explained by a theory model based on the high-order coherent process.

We report the competition between the spontaneous parametric four-wave mixing and secondor fourth-order fluorescence (FL) signals in Pr 3+ :Y 2 SiO 5 crystal. By changing the powers of controlling fields and blocking different fields, the competitive two signals can be identified through the dressing effect. Meanwhile, the delay of fourth-order FL in the time domain results from splitting the energy level. Such results can find potential applications in optical information storage and processing on a photonic chip.

No abstract

Different aspects of the properties of the coexisting super-fluorescence (SFL), multi-wave mixing with the fluorescence signal in the sodium vapor are studied both theoretically and experimentally. First, by scanning the dressed-state, the properties of these coexisting processes, such as the SFL signal modulated by using the dark and bright states, the interplay between dressed-states, are observed for the first time. Then, by scanning the probe field, the interplay between the one-photon and two-photon processes of the coexisting signals is obtained with or without the external dressing fields. Such control on each process in such coexisting system has an important potential application in quantum communication.

We report polarization dressed second-, fourth- and sixth-order fluorescence processes in a Pr(3+):Y2SiO5 crystal. By changing the polarization states of dressing fields and generating fields, the fluorescence baselines, suppression and Autler-Townes splitting of emission peaks can be controlled. The polarization dependencies of fluorescence generated from two inequivalent crystallographic sites are compared. The experimental results agree with the dressing theoretical calculations well.