[1] Atmospheric aerosols represent one of the most important components that attenuate solar radiation reaching the Earth's surface. The aerosol radiative forcing (ARF) at the surface is usually determined in the visible range of the solar spectrum. In contrast, there are few experimental works in the literature about the ARF in the ultraviolet (UV) region. Therefore, this paper focuses on quantifying the aerosol forcing efficiency in the UV erythemal range (AFE ery ), ARF per unit of aerosol optical depth (AOD). Simultaneous UV erythemal irradiance (UVER) and AOD measurements recorded between January 2006 and December 2008 in Granada (Spain) were used. In addition, an empirical model is utilized to estimate the UVER values for an atmosphere with very low aerosol loads (clean conditions). The AFE ery varies from −62 to −26 mW/m 2 per unit of AOD at 380 nm when the solar zenith angle (SZA) changes from 20°to 55°, showing a strong influence of the SZA on AFE ery . The variations of the aerosol size and absorption properties also cause significant changes of this variable. Thus, 1 mm aerosols (related to desert dust particles) produce significantly higher AFE ery (in absolute values) than submicrometer particles (associated with urban or industrial aerosols). For instance, AFE ery varies from −52 mW/m 2 per unit of AOD for Angström exponents smaller than 0.5 to −29 mW/m 2 per unit of AOD for Angström exponents higher than 1.5. In addition, the AFE ery values are −59 mW/m 2 per AOD unit for single-scattering albedos (SSAs) smaller than 0.85 and −28 mW/m 2 per AOD unit for SSAs larger than 0.85, showing that stronger aerosol absorption (low SSA) leads to a larger surface forcing efficiency (in absolute values). All these results highlight the outstanding role that atmospheric aerosol plays in the modifying levels of UV radiation reaching the surface.
This paper presents a study of a strong desert dust episode over the Iberian Peninsula, and its effect on the spectral ultraviolet (UV) irradiance in Granada, Spain. Remote sensing measurements, forecast models, and synoptic analysis are used to identify a Saharan desert dust outbreak that affected the Iberian Peninsula starting 20 July 2009. Additionally, a Bentham DMc150 spectroradiometer is employed to obtain global, direct and diffuse spectral UV irradiances every 15 minutes in Granada. The desert dust caused a large attenuation of the direct UV irradiance (up to 55%), while the diffuse UV irradiance increased up to 40% at 400 nm. The UVSPEC/LibRadtran radiative transfer model is used to study the spectral dependence of the experimental UV irradiance ratios (ratios of spectral irradiance for the day with the highest aerosol load to that measured in days with low–moderate load). The spectral increase or decrease of the UV direct irradiance ratios depends on a new parameter: a threshold wavelength. The spectral dependence of the UV diffuse irradiance ratio can be explained because under the influence of the intense dust outbreak, the Mie scattering by aerosols at shorter wavelengths is stronger than the Rayleigh scattering by gases. Finally, the sensitivity analysis of the aerosol absorption properties shows a substantial attenuation of UV spectral irradiance with a weak spectral dependence
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