The used fuel discharged from nuclear power plants constitutes the main contribution to nuclear waste in countries which do not undertake reprocessing. As such, its disposal requires isolation from the biosphere in stable deep geological formations for long periods of time (some hundred thousand years) until its radioactivity decreases through the process of radioactive decay. Ways for significantly reducing the volumes and radiotoxicities of the waste and to shorten the very long times for which the waste must be stored safely are being investigated. This is the motivation behind the partitioning and transmutation (P&T) activities worldwide. This paper addresses the potential impact of P&T on the long-term disposal of nuclear waste. In particular, it evaluates how realistic P&T scenarios can lead to a reduction in the time required for the waste to be stored safely. The calculations have been done independently by three research groups: ITU and FZK in Germany, and by the CEA in France.

A tuneable ultra-compact high-power, ultra-short pulsed, bright gamma-ray source based on bremsstrahlung radiation from laser-plasma accelerated electrons Novel measurements of electromagnetic radiation above 10 MeV are presented for ultra intense laser pulse interactions with solids. A bright, highly directional source of ␥ rays was observed directly behind the target. The ␥ rays were produced by bremsstrahlung radiation from energetic electrons generated during the interaction. They were measured using the photoneutron reaction ͓ 63 Cu(␥,n) 62 Cu͔ in copper. The resulting activity was measured by coincidence counting the positron annihilation ␥ rays which were produced from the decay of 62 Cu. New measurements of the bremsstrahlung radiation at 10 19 W cm Ϫ2 are also presented.

When a laser pulse of intensity 10(19) W cm(-2) interacts with solid targets, electrons of energies of some tens of MeV are produced. In a tantalum target, the electrons generate an intense highly directional gamma-ray beam that can be used to carry out photonuclear reactions. The isotopes 11C, 38K, (62,64)Cu, 63Zn, 106Ag, 140Pr, and 180Ta have been produced by (gamma,n) reactions using the VULCAN laser beam. In addition, laser-induced nuclear fission in 238U has been demonstrated, a process which was theoretically predicted at such laser intensities more than ten years ago. The ratio of the 11C and the 62Cu beta(+) activities yields shot-by-shot temperatures of the suprathermal electrons at laser intensities of approximately 10(19) W cm(-2).

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Powerful tabletop lasers are now available in the laboratory and can be used to induce nuclear reactions. We report the first demonstration of nuclear fission using a high repetition rate tabletop laser with intensities of 10 20 W/cm 2 . Actinide photo-fission has been achieved in both 238 U and 232 Th from the high-energy bremsstrahlung radiation produced by laser acceleration of electrons. The fission products were identified by time-resolved γspectroscopy.