We present experimental measurements of a pulsed plasma gun, using two-colour imaging laser interferometry and spatially resolved Thomson scattering. Interferometry measurements give an electron density n e ≈ 2.7 × 10 17 cm −3 at the centre of the plasma plume, at 5 mm from the plasma gun nozzle. The Thomson scattered light is collected from two probing angles allowed us to simultaneously measure the collective and non-collective spectrum of the electron feature from the same spatial locations. The inferred electron densities from the location of the electron plasma waves is in agreement with interferometry. The electron temperatures inferred from the two spectra are not consistent, with T e ≈ 10 eV for non-collective scattering and T e ≈ 30 eV for collective scattering. We discuss various broadening mechanisms such as finite aperture effects, density gradients within the collective volume and collisional broadening to account for some of this discrepancy. We also note the significant red/blue asymmetry of the electron plasma waves in the collective scattering spectra, which could relate to kinetic effects distorting the distribution function of the electrons.

The development of versatile nanostructured materials with enhanced nonlinear optical properties is relevant for integrated and energy efficient photonics. In this work, we report third harmonic generation from organic lead...

No abstract

Gallium phosphide (GaP) is a promising material for nanophotonics, given its large refractive index and a transparency over most of the visible spectrum. However, since easy phase‐matching is not possible with bulk GaP, a comprehensive study of its nonlinear optical properties for harmonic generation, especially when grown as thin films, is still missing. Here, second harmonic generation is studied from epitaxially grown GaP thin films, demonstrating that the absolute conversion efficiencies are comparable to a bulk wafer over the pump wavelength range from 1060 to 1370 nm. Furthermore, the results are compared to nonlinear simulations, and the second order nonlinear susceptibility is extracted, showing a similar dispersion and magnitude to that of the bulk material. Furthermore, the third order nonlinear susceptibility of amorphous GaP thin films is extracted from third harmonic generation to be more than one order of magnitude larger than that of the crystalline material, and generation of up to the fifth harmonic is reported. The results show the potential of crystalline and amorphous thin films for nonlinear optics with nanoantennas and metasurfaces, particularly in the visible to near infrared part of the spectrum.

No abstract