Fiber-based light-emitting devices, which can be directly integrated into daily clothes, have emerged as a next-generation display form factor that can provide informational hyper-connections between humans and devices. However, although various approaches have provided advanced wearability, challenges remain for visualizing information, such as high power consumption resulting from high driving voltage and low current efficiency (CE), limited brightness making information difficult to recognize, and lack of addressability for displaying information. Here, a novel fiber-based textile display that can surmount those challenges by successfully introducing phosphorescent organic light-emitting diodes (phOLEDs) based on a dip-coating method and an addressable structure on cylinder-shaped fiber is reported. The fiber phOLEDs exhibit unprecedented optoelectronic performance, including brightness, CE, and driving voltages comparable to those of conventional glass-based OLEDs. Particularly, they show the highest CE values of 16.3, 60.7, and 16.9 cd A -1 for red, green, and blue, respectively, among results reported thus far. Also, the fiber phOLEDs with an addressable structure implementing independent pixels can be operated by the matrix-addressable scheme. Based on unique deformability which is confirmed by flexibility tests, the performance capabilities, and addressability, letter information can be successfully visualized on daily clothes, demonstrating the potential for realizing truly wearable textile displays.
A clothing-type wearable display can be utilized in fashion, bio-healthcare, and safety industries as well as smart textiles for the internet of things (IoTs) and wearable devices. In response to this trend, we demonstrate a textile display that can endure the active movements of a human body. It can be applied to any kind of textile, and is durable against conditions such as rain, sweat, and washing. As a key technology for realizing the multi-directional wrinkle-able textile display, we fabricated a stress-lowering textile platform with an ultrathin planarization layer replicated from the flat surface of glass. An elastomeric strain buffer for reducing mechanical stress is also inserted into the textile platform. Here, organic light-emitting diodes (OLEDs) with red, green and blue color, thin film transistors (TFTs) fabricated at a low temperature below 150 °C, and a washable encapsulation layer blocking both gas and liquid were demonstrated on the textile platform.
The lack of reliable, transparent, and flexible electrodes and insulators for applications in thin-film transistors (TFTs) makes it difficult to commercialize transparent, flexible TFTs (TF-TFTs). More specifically, conventional high process temperatures and the brittleness of these elements have been hurdles in developing flexible substrates vulnerable to heat. Here, we propose electrode and insulator fabrication techniques considering process temperature, transmittance, flexibility, and environmental stability. A transparent and flexible indium tin oxide (ITO)/Ag/ITO (IAI) electrode and an AlO/MgO (AM)-laminated insulator were optimized at the low temperature of 70 °C for the fabrication of TF-TFTs on a polyethylene terephthalate (PET) substrate. The optimized IAI electrode with a sheet resistance of 7 Ω/sq exhibited the luminous transmittance of 85.17% and maintained its electrical conductivity after exposure to damp heat conditions because of an environmentally stable ITO capping layer. In addition, the electrical conductivity of IAI was maintained after 10 000 bending cycles with a tensile strain of 3% because of the ductile Ag film. In the metal/insulator/metal structure, the insulating and mechanical properties of the optimized AM-laminated film deposited at 70 °C were significantly improved because of the highly dense nanolaminate system, compared to those of the AlO film deposited at 70 °C. In addition, the amorphous indium-gallium-zinc oxide (a-IGZO) was used as the active channel for TF-TFTs because of its excellent chemical stability. In the environmental stability test, the ITO, a-IGZO, and AM-laminated films showed the excellent environmental stability. Therefore, our IGZO-based TFT with IAI electrodes and the 70 °C AM-laminated insulator was fabricated to evaluate robustness, transparency, flexibility, and process temperature, resulting in transfer characteristics comparable to those of an IGZO-based TFT with a 150 °C AlO insulator.
We demonstrated that the plasmonic effect can enhance the photoluminescence of the europium organometallic complex in conventional organic light emitting diodes stack from an anode to emissive layer with solution processing. The aggregated gold nanoparticles (A-Au NPs) were incorporated in poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) layer to increase the luminescent quantum efficiency of the emissive layer. An enhancement of 31% was achieved in the emission intensity at 614 nm for samples with A-Au NPs. The reduced exciton lifetime measured by time-resolved photoluminescence comply with the Purcell effect. These improvements are attributed to the localized surface plasmon of A-Au NPs increasing the electric dipole transition rate from Eu 3+ ions.Index Terms-Europium, photoluminescence, plasmons, rare earth metals.
Highly luminescent blue-emitting CdZnS/ZnS nanorods were demonstrated. A study on the electric field-induced fluorescence switching property was presented.
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