A series of experiments is presented which demonstrate significant drag reduction for the laminar flow of water through microchannels using hydrophobic surfaces with well-defined micron-sized surface roughness. These ultrahydrophobic surfaces are fabricated from silicon wafers using photolithography and are designed to incorporate precise patterns of microposts and microridges which are made hydrophobic through a chemical reaction with an organosilane. An experimental flow cell is used to measure the pressure drop as a function of the flow rate for a series of microchannel geometries and ultrahydrophobic surface designs. Pressure drop reductions up to 40% and apparent slip lengths larger than 20 m are obtained using ultrahydrophobic surfaces. No drag reduction is observed for smooth hydrophobic surfaces. A confocal surface metrology system was used to measure the deflection of an air-water interface that is formed between microposts and supported by surface tension. This shear-free interface reduces the flow resistance by allowing the fluid to contact only a very small effective area of the silicon surface. The impact of the surface topology on the drag reduction is explored in detail and the results are found to be in good qualitative agreement with the predictions of analytical theory.
A series of experiments are presented which study the flow kinematics of water past drag-reducing superhydrophobic surfaces. The ultrahydrophobic surfaces are fabricated from silicon wafers using photolithography and are designed to incorporate precise patterns of micrometer-sized ridges aligned in the flow direction. The ridges are made hydrophobic through a chemical reaction with an organosilane. An experimental flow cell is used to measure the velocity profile and the pressure drop as a function of the flow rate for a series of rectangular cross-section microchannel geometries and ultrahydrophobic surface designs. The velocity profile across the microchannel is determined through microparticle image velocimetry ͑-PIV͒ measurements capable of resolving the flow down to lengthscales well below the size of the surface features. Through these detailed velocity measurements, it is demonstrated that slip along the shear-free air-water interface supported between the hydrophobic micrometer-sized ridges is the primary mechanism responsible for the drag reduction observed for flows over ultrahydrophobic surfaces. A maximum slip velocity of more than 60% of the average velocity in the microchannel is found at the center of the shear-free air-water interface whereas the no-slip boundary condition is found to hold along the surface of the hydrophobic ridges. The experimental velocity and pressure drop measurements are compared to the predictions of numerical simulations and an analytical theory based on a simple model of an ultrahydrophobic surface composed of alternating shear-free and no-slip bands with good agreement.
Under laminar, microscale flow conditions, rapid mixing can be difficult to achieve. In these low Reynolds number flows, mixing rates are governed by molecular diffusion, and in the absence of enhanced mixing techniques, mixing lengths and residence times can be much longer than most applications will allow. A number of active mixing techniques have been developed to improve mixing; however, they can be complex to implement and expensive to fabricate. In this paper, we describe a passive mixing method that utilizes a series of ultrahydrophobic surfaces. Our previous experiments have demonstrated that a shear-free air-water interface supported between hydrophobic microridges results in large slip velocities along these ultrahydrophobic surfaces, and significant drag reduction. By aligning the microridges and therefore the air-water interface at an oblique angle to the flow direction, a secondary flow is generated, which is shown to efficiently stretch and fold the fluid elements and reduce the mixing length by more than an order of magnitude compared to that of a smooth microchannel. The designs of the ultrahydrophobic surfaces were optimized through experiments and numerical simulations. A Y-shaped channel was used to bring two streams of water together, one tagged with a fluorescent dye. A confocal microscope was used to measure fluorescence intensity and dye concentration. Quantitative agreement between the experiments and the numerical simulations was achieved for both the flow patterns and degree of mixing. Increasing the angle of the microridges was found to reduce the mixing length up to a critical angle of about 60 degrees , beyond which the mixing length was found to increase with further increases to the angle of the microridge. The mixing enhancement was found to be much less sensitive to changes in microridge width or separation.
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