Scattering-type scanning near-field optical microscopy (SNOM) offers the possibility to analyze material properties like strain in crystals at the nanoscale. In this paper we introduce a SNOM setup employing a newly developed tunable broadband laser source with a covered spectral range from 9 µm to 16 µm. This setup allows for the first time optical analyses of the crystal structure of gallium nitride (GaN) at the nanometer scale by excitation of a near-field phonon resonance around 14.5 µm. On the example of an artificially induced stress field within a GaN wafer, we present a method for a 2D visualization of small deviations in the crystal structure, which allows for fast qualitative characterizations. Subsequently, the stress levels at chosen points were quantified by recording complex near-field spectra and correlating them with theoretical model calculations. Applied to the cross-section of a heteroepitaxially grown GaN wafer, we finally demonstrate the capability of our setup to analyze the relaxation of the crystal structure along the growth axis with a nanometer spatial resolution.

Abstract. In the field of atmospheric research, lidar is a powerful technology that can measure gas or aerosol concentrations, wind speed, or temperature profiles remotely. To conduct such measurements globally, spaceborne systems are advantageous. Pulse energies in the 100-mJ range are required to achieve highly accurate, longitudinal resolved measurements. Measuring concentrations of specific gases, such as CH 4 or CO 2 , requires output wavelengths in the IR-B, which can be addressed by optical-parametric frequency conversion. An OPO/ OPA frequency conversion setup was designed and built as a demonstration module to address the 1.6-μm range. The pump laser is an Nd:YAG-MOPA system, consisting of a stable oscillator and two subsequent Innoslab-based amplifier stages that deliver up to 500 mJ of output pulse energy at 100 Hz repetition frequency. The OPO is inherited from the OPO design for the CH 4 lidar instrument on the French-German climate satellite methane remote-sensing lidar mission (MERLIN). To address the 100-mJ regime, the OPO output beam is amplified in a subsequent multistage OPA. With potassium titanyl phosphate as nonlinear medium, the OPO/OPA delivered more than 100 mJ of output energy at 1645 nm from 450 mJ of the pump energy and a pump pulse duration of 30 ns. This corresponds to a quantum conversion efficiency of about 25%. In addition to demonstrating optical performance for future lidar systems, this laser will be part of a laser-induced damage thresholds test facility, which will be used to qualify optical components especially for the MERLIN. © The Authors.Published by SPIE under a Creative Commons Attribution 3.0 Unported License. Distribution or reproduction of this work in whole or in part requires full attribution of the original publication, including its DOI.

We present a theoretical and experimental analysis of a pulsed 1645 nm optical parametric oscillator (OPO) to prove the feasibility of such a device for a spaceborne laser transmitter in an integrated path differential absorption (IPDA) lidar system. The investigation is part of the French-German satellite mission MERLIN (Methane Remote Sensing Lidar Mission). As an effective greenhouse gas, methane plays an important role for the global climate. The architecture of the OPO is based on a conceptual design developed by DLR, consisting of two KTA crystals in a four-mirror-cavity. Using numerical simulations, we studied the performance of such a setup with KTP and investigated means to optimize the optical design by increasing the efficiency of the OPO and decreasing the fluence on the optical components. For the experimental testing of the OPO, we used the INNOSlab-based ESA pre-development model ATLAS as pump laser at 1064 nm. The OPO obtained 9.2 mJ pulse energy at 1645 nm from 31.5 mJ of the pump and a pump pulse duration of 42 ns. This corresponds to an optical/optical efficiency of 29%. After the pump pulse was reduced to 24 ns, a similar OPO performance could be obtained by adapting the pump beam radius. In recent experiments with optimized optical design the OPO obtained 12.5 mJ pulse energy at 1645 nm from 32.0 mJ of the pump, corresponding to an optical/optical efficiency of 39%. Two different methods were applied to study the laser damage thresholds of the optical elements used

We present a theoretical and experimental analysis of a pulsed 1645 nm optical parametric oscillator (OPO) conducted to prove the feasibility of such a device for a spaceborne laser transmitter in an integrated path differential absorption (IPDA) lidar system. The investigation is part of the French-German satellite mission MERLIN (Methane Remote Sensing Lidar Mission). As an effective greenhouse gas, methane plays an important role for the global climate.The architecture of the OPO is based on a conceptual design developed by DLR, consisting of two KTA crystals in a four-mirror-cavity. One of the cavity mirrors is piezo-driven to provide single frequency operation of the OPO. Using numerical simulations, we studied the performance and alignment tolerances of such a setup with KTP and KTA and investigated means to optimize the optical design by increasing the efficiency and decreasing the fluence on the optical components. For the experimental testing of the OPO, we used the INNOSlab-based ESA pre-development model ATLAS as pump laser at 1064 nm. At a pulse frequency of 25 Hz this MOPA delivers a pump energy up to 45 mJ with a beam quality factor of about M² = 1.3. With KTP as nonlinear crystal the OPO obtained 9.2 mJ pulse energy at 1645 nm from 31.5 mJ of the pump and a pump pulse duration of 42 ns. This corresponds to an optical/optical efficiency of 29%. After the pump pulse was reduced to 24 ns a similar OPO performance could be obtained by adapting the pump beam radius.

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