We demonstrate how to suspend various magnetic and non-magnetic particles in liquid metals and characterize their properties relevant to magnetohydrodynamics (MHD). The suspending method uses an acid as a flux to eliminate oxidation from both metal particles and liquid, which allows the particles to be wetted and suspend into the liquid if the particles have higher conductivity than the liquid. With this process we were able to suspend a wide range of particle materials and sizes from 40 nm to 500 µm, into three different liquid metal bases, and volume fractions φ up to the liquid-solid transition φc. By controlling the volume fraction of iron particles in liquid eGaIn, we increased the magnetic permeability by a factor of 5.0 and the electrical conductivity by 13% over that of the pure liquid metal, which gives these materials the potential to exhibit strong MHD effects on the laboratory scale that are usually only observable in the cores of planets and stars. By adding non-magnetic zinc particles, we increased the viscosity by a factor of 160 while keeping the magnetic and electrical properties nearly constant, which would allow independent control of MHD effects from turbulence. We show that the suspensions flow like Newtonian fluids up to the volume fraction of the liquid-solid transition φc.
We demonstrate strain-induced coupling between a hole spin in a quantum dot and mechanical motion of a cantilever. The optical transitions of quantum dots integrated into GaAs mechanical resonators are measured synchronously with the motion of the driven resonators. In a Voigt magnetic field, both electron and hole spin splittings are measured, showing negligible change for the electron spin but a large change for the hole spin of up to 36%. This large effect is attributed to the stronger spin orbit interaction of holes compared to electrons.
A variety of quantum degrees of freedom, e.g., spins, valleys, and localized emitters, in atomically thin van der Waals materials have been proposed for quantum information applications, and they inevitably couple to phonons. Here, we directly measure the intrinsic optical phonon decoherence in monolayer and bulk MoS 2 by observing the temporal evolution of the spectral interference of Stokes photons generated by pairs of laser pulses. We find that a prominent optical phonon mode E 2g exhibits a room-temperature dephasing time of ∼7 ps in both the monolayer and bulk. This dephasing time extends to ∼20 ps in the bulk crystal at ∼15 K, which is longer than previously thought possible. Firstprinciples calculations suggest that optical phonons decay via two types of three-phonon processes, in which a pair of acoustic phonons with opposite momentum are generated.
We characterize how suspensions of magnetic particles in a liquid respond to a magnetic field in terms of the effective magnetic susceptibility χ ef f using inductance measurements. We test a model that predicts how χ ef f varies due to demagnetization, as a function of sample aspect ratio, particle packing fraction, and particle aspect ratio [1]. For spherical particles or cylindrical particles aligned with external magnetic field, the model can be fitted to the measured data with agreement within 17%. However, we find that the random alignment of particles relative to the magnetic field plays a role, reducing χ ef f by a factor of 3 in some cases, which is not accounted for in models yet. While suspensions are predicted to have χ ef f that approach the particle material susceptibility in the limit of large particle aspect ratio, instead we find a much smaller particle aspect ratio where χ ef f is maximized. A prediction that χ ef f approaches the bulk material susceptibility in the limit of the packing fraction of the liquid-solid transition also fails. We find χ ef f no larger than about 4 for suspensions of iron particles.
High resolution optical spectroscopy methods are demanding in terms of either technology, equipment, complexity, time or a combination of these. Here we demonstrate an optical spectroscopy method that is capable of resolving spectral features beyond that of the spin fine structure and homogeneous linewidth of single quantum dots (QDs) using a standard, easy-to-use spectrometer setup. This method incorporates both laser and photoluminescence spectroscopy, combining the advantage of laser line-width limited resolution with multi-channel photoluminescence detection. Such a scheme allows for considerable improvement of resolution over that of a common single-stage spectrometer. The method uses phonons to assist in the measurement of the photoluminescence of a single quantum dot after resonant excitation of its ground state transition. The phonon's energy difference allows one to separate and filter out the laser light exciting the quantum dot. An advantageous feature of this method is its straight forward integration into standard spectroscopy setups, which are accessible to most researchers.
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