We present experimental and theoretical results on high-harmonic generation in noble gases using an 805 nm, 25 fs, titanium-doped sapphire laser. The harmonic energies observed are unexpectedly high when compared with experimental and theoretical results to date for longer excitation pulses. We observe that the efficiency of harmonic production is highest for shorter pulses. Furthermore, the wavelength of the harmonics can be tuned by adjusting the sign of the chirp of the excitation pulse, demonstrating a tunable, ultrashort-pulse, ,25 fs soft-x-ray source.
An improved approach to assemble ultrathin and thickness-tunable polypyrrole (PPy) films onto multiwall carbon nanotubes (MWCNTs) has been investigated. A facile procedure is demonstrated for controlling the morphology and thickness of PPy film by adding ethanol in the reaction system and a possible mechanism of the coating formation process is proposed. The coated PPy films can be easily tuned by adding ethanol and adjusting a mass ratio of pyrrole to MWCNTs. Moreover, the thickness of PPy significantly influences the electronic conductivity and capacitive behavior of the PPy/MWCNT composites. The method may provide a facile strategy for tailoring the polymer coating on carbon nanotubes (CNTs) for carbon-based device applications.
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