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In preparation of a laser ion source, we have investigated multi-step laser ionization via Rydberg and autoionizing states for atomic Ni and Ge using a mass separator with an ion beam energy of 20 keV. For both elements resonant three-step excitation schemes suitable for modern Ti:sapphire laser systems were developed. Rydberg series in the range of principal quantum numbers 20 n 80 were localized, assigned and quantum numbers were allocated to the individual resonances. Ionization potentials (IP) were extracted from fits of the individual series and quantum defects of individual levels were analysed for confirmation of series assignment. For Ni the ionization potential could be extracted with significantly increased precision compared to literature with a value of E IP (Ni) = 61 619.77(14) cm −1. Also, at least one notable autoionizing state above the first IP was discovered for both elements, and the different ionization schemes via Rydberg or autoionizing states were compared with respect to line shape, ionization efficiency and selectivity.

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A new type of resonance ionization laser ion source (RILIS) is presently being developed and tested at the off-line mass separator at Mainz University for future use at on-line exotic rare isotopes production facilities. For highest isobaric selectivity, this RILIS approach decouples the evaporation and ionization process. A further advantage is the generation of full temporal control of the resulting high quality ion beam. These facts are realized by a combination of atomizer -ion repeller -ion cooler and trap, which is operated together with a state-of-the-art, all solid state laser system. The principle and performance of this laser ion source trap (LIST) system are discussed applying simulation studies for the repeller-trap combination and first measurements for characterization.

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