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The authors report on high quality ZnCdO alloy epilayers and ZnCdO/ZnO single quantum well structures on sapphire substrates by pulsed laser deposition. The Cd concentration in the ZnCdO alloy can be systematically adjusted via the substrate temperature and single-phase ZnCdO alloy with a band gap at room temperature extended to 2.94 eV is achieved. The single quantum well structures exhibit strong photoluminescence from the well layer with extremely weak emission from deep level defects and the ZnO barrier, indicating the high quality of ZnCdO/ZnO single quantum well structures.
We present on a systematic study of the contribution of surface plasmon (SP) coupling and light extraction toward emission enhancement of Platinum (Pt) nano-patterns capped MgZnO films. Time resolved Photoluminescence (PL) results indicate that the Pt coating can greatly reduces the non-radiative recombination rate by passivation of surface states, making the decay slow down. Temperature dependence of the integrated photoluminescence intensity reveals that the Pt nano-patterns can offer a large amount of light transfer and scattering, which enormously increase the light extraction efficiency up to 3.8-fold. These results indicate that the increased light extraction efficiency caused by surface modification via Pt coating rather than SP coupling plays a dominant role in increasing bandgap emission of MgZnO film.
We present our study of the dependence of surface plasmon (SP) coupled band gap emission and defect emission on the sputtering time of gold particles on ZnCdO films. Eightfold enhancement of the band gap emission from ZnCdO thin films coated with Au particles is observed, while the defect emission is completely suppressed. The remarkable enhancement of the band gap emission is mainly attributed to the coupling between excitons in ZnCdO films and the SP of Au particles. While the suppression of the defect emission may be ascribed to a combined effect of the reduction in surface defects and the charge transfer from defect level to the Au Fermi level.
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