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In this work, we present a suitable material for metal-based spin-valve in current-perpendicular-to-plane (CPP) geometry. The AΔR (A is the element size and ΔR is the change in resistance) was investigated for three kinds of free and pinned layers material, that is, Co90Fe10, Fe50Co50, and Fe50Co50 with half-atomic Cu layers. When the free and pinned layers are 5 nm, AΔR is 1.0 mΩ μm2, 1.6 mΩ μm2, and 2.9 mΩ μm2, respectively. Moreover, the dual-type spin valve having Fe50Co50 with half-atomic Cu layers achieved 5.2 mΩ μm2. According to the free and pinned layers thickness dependence of AΔR, the spin-dependent resistance at the interfaces between ferromagnetic layers and spacer Cu is enhanced mainly by changing from Co90Fe10 to Fe50Co50, and the spin-dependent bulk resistance in free and pinned layers is enlarged by inserting half-atomic Cu layers.

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