Understanding the fracture toughness (resistance) of glasses is a fundamental problem of prime theoretical and practical importance. Here we theoretically study its dependence on the loading rate, the age (history) of the glass and the notch radius ρ. Reduced-dimensionality analysis suggests that the notch fracture toughness results from a competition between the initial, age-and historydependent, plastic relaxation timescale τ pl 0 and an effective loading timescale τ ext (KI , ρ), whereKI is the tensile stress-intensity-factor rate. The toughness is predicted to scale with √ ρ independentlypl 0 for ξ 1, to scale as T √ ρ log(ξ) for ξ 1 (related to thermal activation, where T is the temperature) and to feature a non-monotonic behavior in the crossover region ξ ∼ O(1) (related to plastic yielding dynamics). These predictions are verified using novel 2D computations, providing a unified picture of the notch fracture toughness of glasses. The theory highlights the importance of timescales competition and far from steady-state elasto-viscoplastic dynamics for understanding the toughness, and shows that the latter varies quite significantly with the glass age (history) and applied loading rate. Experimental support for bulk metallic glasses is presented.
Crack pinning by heterogeneities is a central toughening mechanism in the failure of brittle materials. So far, most analytical explorations of the crack front deformation arising from spatial variations of fracture properties have been restricted to weak toughness contrasts using first order approximation and to defects of small dimensions with respect to the sample size. In this work, we investigate the non-linear effects arising from larger toughness contrasts by extending the approximation to the second order, while taking into account the finite sample thickness. Our calculations predict the evolution of a planar crack lying on the mid-plane of a plate as a function of the material parameters and the loading conditions, especially in the case of a single infinitely elongated obstacle. Peeling experiments are presented which validate the approach and evidence that the second order term broadens its range of validity in terms of toughness contrast values. The work highlights the non-linear response of the crack front to strong defects and the central role played by the thickness of the specimen on the pinning process.
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