Interacting Bosons in artificial lattices have emerged as a modern platform to explore collective manybody phenomena and exotic phases of matter as well as to enable advanced on-chip simulators. On chip, exciton–polaritons emerged as a promising system to implement and study bosonic non-linear systems in lattices, demanding cryogenic temperatures. We discuss an experiment conducted on a polaritonic lattice at ambient conditions: We utilize fluorescent proteins providing ultra-stable Frenkel excitons. Their soft nature allows for mechanically shaping them in the photonic lattice. We demonstrate controlled loading of the coherent condensate in distinct orbital lattice modes of different symmetries. Finally, we explore the self-localization of the condensate in a gap-state, driven by the interplay of effective interaction and negative effective mass in our lattice. We believe that this work establishes organic polaritons as a serious contender to the well-established GaAs platform for a wide range of applications relying on coherent Bosons in lattices.
The strong light-matter coupling of a microcavity mode to tightly bound Frenkel excitons in organic materials emerged as a versatile, room-temperature compatible platform to study nonlinear many-particle physics and bosonic condensation. However, various aspects of the optical response of Frenkel excitons in this regime remained largely unexplored. Here, we utilize a hemispheric optical cavity filled with the fluorescent protein mCherry to address two important questions in the field of room-temperature polariton condensates. First, combining the high quality factor of the microcavity with a well-defined mode structure allows us to provide a definite answer whether temporal coherence in such systems can become competitive with their low-temperature counterparts. We observe highly monochromatic and coherent light beams emitted from the condensate, characterized by a coherence time greater than 150 ps, which exceeds the polariton lifetime by two orders of magnitude. Second, the high quality of our device allows to sensibly trace the emission energy of the condensate, and thus to establish a fundamental picture which quantitatively explains the core nonlinear processes yielding the characteristic density-dependent blueshift. We find that the energy shift of Frenkel excitonpolaritons is largely dominated by the reduction of the Rabi-splitting due to phase space filling effects, which is influenced by the redistribution of polaritons in the system. While our finding of highly coherent condensation at ambient conditions addresses the suitability of organic polaritonics regarding their utilization as highly coherent room temperature polariton lasers, shedding light on the non-linearity is of great benefit towards implementing non-linear devices, optical switches, and lattices based on exciton-polaritons at room temperature.
Interacting bosonic particles in artificial lattices have proven to be a powerful tool for the investigation of exotic phases of matter as well as phenomena resulting from non-trivial topology. Exciton-polaritons, bosonic quasi-particles of light and matter, have shown to combine the on-chip benefits of optical systems with strong interactions, inherited form their matter character. Technologically significant semiconductor platforms, however, strictly require cryogenic temperatures for operability. In this paper, we demonstrate exciton-polariton lasing for topological defects emerging form the imprinted lattice structure at room temperature. We utilize a monomeric red fluorescent protein derived from DsRed of Discosoma sea anemones, hosting highly stable Frenkel excitons. Using a patterned mirror cavity, we tune the lattice potential landscape of a linear Su-Schrieffer-Heeger chain to design topological defects at domain boundaries and at the edge. In spectroscopic experiments, we unequivocally demonstrate polariton lasing from these topological defects. This progress promises to be a paradigm shift, paving the road to interacting Boson many-body physics at ambient conditions.
Engineering non-linear hybrid light-matter states in tailored lattices is a central research strategy for the simulation of complex Hamiltonians. Excitons in atomically thin crystals are an ideal active medium for such purposes, since they couple strongly with light and bear the potential to harness giant non-linearities and interactions while presenting a simple sample-processing and room temperature operability. We demonstrate lattice polaritons, based on an open, high-quality optical cavity, with an imprinted photonic lattice strongly coupled to excitons in a WS2 monolayer. We experimentally observe the emergence of the canonical band-structure of particles in a one-dimensional lattice at room temperature, and demonstrate frequency reconfigurability over a spectral window exceeding 85 meV, as well as the systematic variation of the nearest-neighbour coupling, reflected by a tunability in the bandwidth of the p-band polaritons by 7 meV. The technology presented in this work is a critical demonstration towards reconfigurable photonic emulators operated with non-linear photonic fluids, offering a simple experimental implementation and working at ambient conditions.
Applications that require the measurement of the spatially averaged velocity over a given area segment can be addressed by the thermal transient anemometer (TTA). The operating principle can be characterized as follows: (i) elevate the temperature of the multi-X patterned sensor—that appropriately samples the area of interest—to an initial overheat condition, (ii) allow the sensor to cool by the heat transfer of the passing fluid (plus end conduction effects), (iii) execute a calibration such that the exponential decay of the sensor resistance can be characterized by the time constant, τ, and (iv) infer the spatially averaged velocity ⟨U⟩—or the spatially averaged density–velocity product ⟨ρU⟩—from the relationship Note that A″, B″, n are defined by the calibration data. A description of the enabling electronics, demonstration measurements in a calibration air stream and the post-processing strategy to account for ambient temperature changes between calibration and test data are presented in order to characterize this instrument.
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