This work demonstrates a stretchable and flexible lactate/O 2 biofuel cell (BFC) using buckypaper (BP) composed of multi-walled carbon nanotubes (MWCNTs) as the electrode material. Free-standing BP, functionalized with a pyrene-polynorbornene homopolymer, is fabricated as the immobilization matrix for lactate oxidase (LOx) at the anode and bilirubin oxidase (BOx) at the cathode. This biofuel cell delivers an open circuit voltage of 0.74 V and a high-power density of 520 µW cm-2. The functionalized BP electrodes are assembled onto a stretchable screen-printed current collector with an "island-bridge" configuration, which ensures conformal contact between the wearable BFC and the This article is protected by copyright. All rights reserved. 2 human body and endows the BFC with excellent performance stability under stretching condition. When applied to the arm of the volunteer, the BFC can generate a maximum power of 450 µW. When connected with a voltage booster, the on-body BFC is able to power a light emitting diode under both pulse discharge and continuous discharge modes during exercise. This demonstrates the promising potential of the flexible BP-based BFC as a self-sustained power source for next generation wearable electronics. Received: ((will be filled in by the editorial staff)) Revised: ((will be filled in by the editorial staff))
This work demonstrates the first example of sweat-based wearable and stretchable biosupercapacitors (BSCs), capable of generating high-power pulses from human activity. The all-printed, dual-functional, conformal BSC platform can harvest and store energy from sweat lactate. By integrating energy harvesting and storage functionalities on the same footprint of a single epidermal device, the new wearable energy system can deliver highpower pulses and be rapidly self-charged by bioenergy conversion of sweat lactate generated from human activity while simplifying the design and fabrication. The mechanical robustness and conformability of the device are realized through island-bridge patterns and strain-enduring inks. The enhanced capacitance of the BSC is realized by the synergistic effect of carbon nanotube ink with electrodeposited polypyrrole on the anode and of porous cauliflowerlike platinum on the cathode. In the presence of lactate, the BSC shows high power in pulsed output and stable cycling performance. Furthermore, the wearable device can store energy and deliver high-power pulses long after the perspiration stopped. The self-charging hybrid wearable device obtained high power of 1.7 mW cm −2 in vitro, and 343 µW cm −2 on the body during exercise, suggesting considerable potential as a power source for the next generation of wearable electronics.
Memetic Algorithms (MAs) represent an emerging field that has attracted increasing research interest in recent times. Despite the popularity of the field, we remain to know rather little of the search mechanisms of MAs. Given the limited progress made on revealing the intrinsic properties of some commonly used complex benchmark problems and working mechanisms of Lamarckian memetic algorithms in general non-linear programming, we introduce in this work for the first time the concepts of local optimum structure and generalize the notion of neighborhood to connectivity structure for analysis of MAs. Based on the two proposed concepts, we analyze the solution quality and computational efficiency of the core search operators in Lamarckian memetic algorithms. Subsequently, the structure of local optimums of a few representative and complex benchmark problems is studied to reveal the effects of individual learning on fitness landscape and to gain clues into the success or failure of MAs. The connectivity structure of local optimum for different memes or individual learning procedures in Lamarckian MAs on the benchmark problems is also investigated to understand the effects of choice of memes in MA design. = Conditional probability density function of having offspring y given parent x at generation
A novel wideband circularly polarized antenna array using sequential rotation feeding network is presented in this paper. The proposed antenna array has a relative bandwidth of 38.7% at frequencies from 5.05 GHz to 7.45 GHz with a highest gain of 12 dBi at 6 GHz. A corresponding left-handed metamaterial is designed in order to increase antenna gain without significantly affecting its polarization characteristics. The wideband circularly polarized antenna with 2.4 GHz of bandwidth is a promising solution for wireless communication system such as tracking or wireless energy harvesting from Wi-Fi signal based on IEEE 802.11ac standard or future 5G cellular. A potential application of this antenna as a receiving antenna for RF-DC device to obtain DC power for a wireless sensor node from Wi-Fi signal is shown.
Nanoporous SnO2 thin films were elaborated to serve as sensing electrodes for label-free DNA detection using electrochemical impedance spectroscopy (EIS). Films were deposited by an electrodeposition process (EDP). Then the non-Faradic EIS behaviour was thoroughly investigated during some different steps of functionalization up to DNA hybridization. The results have shown a systematic decrease of the impedance upon DNA hybridization. The impedance decrease is attributed to an enhanced penetration of ionic species within the film volume. Besides, the comparison of impedance variations upon DNA hybridization between the liquid and vapour phase processes for organosilane (APTES) grafting on the nanoporous SnO2 films showed that vapour-phase method is more efficient. This is due to the fact that the vapour is more effective than the solution in penetrating the nanopores of the films. As a result, the DNA sensors built from vapour-treated silane layer exhibit a higher sensitivity than those produced from liquid-treated silane, in the range of tested target DNA concentration going to 10 nM. Finally, the impedance and fluorescence response signals strongly depend on the types of target DNA molecules, demonstrating a high selectivity of the process on nanoporous SnO2 films.
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