Microresonator frequency combs based on the χ(3) nonlinearity are nowadays well understood and making their way into different applications. Recently, microresonator frequency combs based on the χ(2) nonlinearity are receiving increasing attention, as they promise certain benefits, but still require further study. Here, we present the first indication of χ(2) frequency comb generation, initiated via optical parametric oscillation (OPO) in a lithium niobate mm-sized microresonator. By pumping at 532 nm with 300 µW of power, we observe 1-THz-wide comb spectra around 1064 nm with degenerate and non-degenerate states. We also show that comb generation requires signal and idler waves to be degenerate in mode numbers and how the fulfillment of this condition can be identified from the temperature tuning curves. The results demonstrate the potential to directly generate frequency combs via OPO beyond 3 μm wavelengths in the mid-IR by puming in the near-IR region.

Owing to the discrete frequency spectrum of whispering gallery resonators (WGRs), the resonance and phase-matching conditions for the interacting waves in the case of second-harmonic generation (SHG) cannot generally be fulfilled simultaneously. To account for this, we develop a model describing SHG in WGRs with non-zero frequency detunings at both the pump and second-harmonic frequencies. Our model predicts strong distortions of the line shape of pump and second-harmonic resonances for similar linewidths at both frequencies; for much larger linewidths at the second-harmonic frequency, this behavior is absent. Furthermore, it describes the SHG efficiency as a function of detuning. Experimentally, one can change the WGR eigenfrequencies, and thus the relative detuning between pump and second-harmonic waves by a number of means, for example electro-optically and thermally. Using a lithium niobate WGR, we show an excellent quantitative agreement for the SHG efficiency between our experimental results and the model. Also, we show the predicted distortions of the pump and second-harmonic resonances to be absent in the lithium niobate WGR but present in a cadmium silicon phosphide WGR, as expected from the linewidths of the resonances involved.

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Optical parametric oscillators (OPOs) constitute an important coherent, narrow-linewidth and widely tunable light source with applications in spectroscopy and many other fields. Their realizations based on whispering gallery resonators (WGRs) provide a small footprint and ultra-low thresholds, with demonstrations of tunability typically done via temperature variation. In this work, we show the pump tuning capabilities of a mm-sized WGR mid-infrared OPO made of CdSiP2. By tuning a telecom wavelength diode laser by 16 nm, we generate tunable light from 2708 to 3575 nm. Furthermore, we show controlled tuning in steps of 1 free spectral range (FSR) and the possibility of 12 GHz of continuous tuning. All these features are in good agreement with the theoretical predictions. We conclude that tuning from 2.4 to 4.9 µm is even possible, while still using commercially available near-infrared diode lasers. This work highlights the advantages of pump tuning of WGR OPOs and provides valuable insights for their precise control.

The potential of frequency comb spectroscopy has aroused great interest in generating mid-infrared frequency combs in the integrated photonic setting. However, despite remarkable progress in microresonators and quantum cascade lasers, the availability of suitable mid-IR comb sources remains scarce. Here, we generate mid-IR microcombs relying on cascaded three-wave-mixing for the first time. By pumping a CdSiP2 microresonator at 1.55 µm wavelength with a low power continuous wave laser, we generate χ(2) frequency combs at 3.1 µm wavelength, with a span of about 30 nm. We observe ordinary combs states with a line spacing of the free spectral range of the resonator, and combs where the sideband numbers around the pump and half-harmonic alternate, forming staggered patterns of spectral lines. Our scheme for mid-IR microcomb generation is compatible with integrated telecom lasers. Therefore, it has the potential to be used as a simple and fully integrated mid-IR comb source, relying on only one single material.