We show, both theoretically and experimentally, that high-numerical-aperture (NA) optical microscopy is accompanied by strong spin-orbit interaction of light, which translates fine information about the specimen to the polarization degrees of freedom of light. An 80 nm gold nanoparticle scattering the light in the focus of a high-NA objective generates angular momentum conversion, which is seen as a nonuniform polarization distribution at the exit pupil. We demonstrate remarkable sensitivity of the effect to the position of the nanoparticle: Its subwavelength displacement produces the giant spin-Hall effect, i.e., macroseparation of spins in the outgoing light. This brings forth a far-field optical nanoprobing technique based on the spin-orbit interaction of light.
We present a general theory of spin-to-orbital angular momentum (AM) conversion of light in focusing, scattering, and imaging optical systems. Our theory employs universal geometric transformations of non-paraxial optical fields in such systems and allows for direct calculation and comparison of the AM conversion efficiency in different physical settings. Observations of the AM conversions using local intensity distributions and far-field polarimetric measurements are discussed.
We show that, in order to attain complete polarization control across a beam, two spatially resolved variable retardations need to be introduced to the light beam. The orientation of the fast axes of the retarders must be linearly independent on the Poincaré sphere if a fixed starting polarization state is used, and one of the retardations requires a range of 2π. We also present an experimental system capable of implementing this concept using two passes on spatial light modulators (SLMs). A third SLM pass can be added to control the absolute phase of the beam. Control of the spatial polarization and phase distribution of a beam has applications in high-NA microscopy, where these properties can be used to shape the focal field in three dimensions. We present some examples of such fields, both theoretically calculated using McCutchen's method and experimentally observed.
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