The new‐generation polar‐orbiting operational environmental sensor, the Visible Infrared Imaging Radiometer Suite (VIIRS) on board the Suomi National Polar‐orbiting Partnership (S‐NPP) satellite, provides critical daily global aerosol observations. As older satellite sensors age out, the VIIRS aerosol product will become the primary observational source for global assessments of aerosol emission and transport, aerosol meteorological and climatic effects, air quality monitoring, and public health. To prove their validity and to assess their maturity level, the VIIRS aerosol products were compared to the spatiotemporally matched Aerosol Robotic Network (AERONET) measurements. Over land, the VIIRS aerosol optical thickness (AOT) environmental data record (EDR) exhibits an overall global bias against AERONET of −0.0008 with root‐mean‐square error (RMSE) of the biases as 0.12. Over ocean, the mean bias of VIIRS AOT EDR is 0.02 with RMSE of the biases as 0.06. The mean bias of VIIRS Ocean Ångström Exponent (AE) EDR is 0.12 with RMSE of the biases as 0.57. The matchups between each product and its AERONET counterpart allow estimates of expected error in each case. Increased uncertainty in the VIIRS AOT and AE products is linked to specific regions, seasons, surface characteristics, and aerosol types, suggesting opportunity for future modifications as understanding of algorithm assumptions improves. Based on the assessment, the VIIRS AOT EDR over land reached Validated maturity beginning 23 January 2013; the AOT EDR and AE EDR over ocean reached Validated maturity beginning 2 May 2012, excluding the processing error period 15 October to 27 November 2012. These findings demonstrate the integrity and usefulness of the VIIRS aerosol products that will transition from S‐NPP to future polar‐orbiting environmental satellites in the decades to come and become the standard global aerosol data set as the previous generations' missions come to an end.

[1] The GOES Aerosol/Smoke Product (GASP) is a retrieval of the aerosol optical depth (AOD) using visible imagery. The product currently runs operationally at NOAA/NESDIS in near-real time at 30 min intervals. This high temporal resolution is not possible with polar orbiting instruments which produce one daily image. This work evaluates the GASP AOD from the GOES-12 Imager over North America at various temporal and spatial scales based on comparisons with AOD from the Aerosol Robotic Network (AERONET) and the Moderate Resolution Imaging Spectroradiometer (MODIS). We find a mean GASP/AERONET correlation of 0.79, rms difference of 0.13 and slope of 0.8, based on a statistical analysis at 10 northeastern U.S. and Canadian sites. The GASP AOD has a slight negative bias when the AOD is greater than 0.35 and a positive bias elsewhere. The absolute bias is less than 30% when the AOD is greater than 0.1. When the AOD is less than 0.15 we find poor correlation and biases greater than 30%. The GASP/ AERONET statistics also indicate that GASP can be used to examine the seasonal and diurnal variability in the AOD over the eastern United States between 1215 and 2115 UTC. GASP/AERONET AOD correlations were generally less than 0.5 elsewhere in the continental United States. Comparisons between the MODIS and GASP AOD over the eastern United States in the summer of 2004 showed agreement within 20% and correlations greater than 0.7 under elevated AOD conditions. Simultaneous comparisons between GASP, MODIS, and AERONET AODs showed good agreement over the northeastern United States and Canada, with higher correlation and lower rms differences in the MODIS/AERONET comparisons than in the GASP/AERONET comparisons.