We study theoretically the generation of photon pairs by spontaneous four-wave mixing (SFWM) in photonic crystal optical fiber. We show that it is possible to engineer two-photon states with specific spectral correlation ("entanglement") properties suitable for quantum information processing applications. We focus on the case exhibiting no spectral correlations in the two-photon component of the state, which we call factorability, and which allows heralding of single-photon pure-state wave packets without the need for spectral post filtering. We show that spontaneous four wave mixing exhibits a remarkable flexibility, permitting a wider class of two-photon states, including ultra-broadband, highly-anticorrelated states.

We present the implementation of a combined digital scanned light-sheet microscope (DSLM) able to work in the linear and nonlinear regimes under either Gaussian or Bessel beam excitation schemes. A complete characterization of the setup is performed and a comparison of the performance of each DSLM imaging modality is presented using in vivo Caenorhabditis elegans samples. We found that the use of Bessel beam nonlinear excitation results in better image contrast over a wider field of view.

We study the process of co-polarized spontaneous four-wave mixing in single-mode optical fibers, with an emphasis on an analysis of the conversion efficiency. We consider both the monochromaticpumps and pulsed-pumps regimes, as well as both the degenerate-pumps and non-degenerate-pumps configurations. We present analytical expressions for the conversion efficiency, which are given in terms of double integrals. In the case of pulsed pumps we take these expressions to closed analytical form with the help of certain approximations. We present results of numerical simulations, and compare them to values obtained from our analytical expressions, for the conversion efficiency as a function of several key experimental parameters.

The third-order nonlinear optical response of a thin film containing the azobenzene dye Disperse Red 1 was studied using the z-scan technique with tunable picosecond pulses. A nonlinear refractive index of −5.0 cm2/GW, corresponding to a Re χ(3)=−3.0×10−15 m2/V2 (2.1×10−7 esu), has been measured at 570 nm. The observed nonlinearity is attributed to the change in refractive index induced by the trans-cis transition in the dye molecule.

We present a study of the spectral properties of photon pairs generated through the process of spontaneous four wave mixing (SFWM) in single mode fiber. Our analysis assumes narrowband pumps, which are allowed to be frequency-degenerate or non-degenerate. Based on this analysis, we derive conditions on the pump frequencies and on the fiber dispersion parameters which guarantee the generation of ultra-broadband photon pairs. Such photon pairs are characterized by: i) a very large degree of entanglement, and ii) a very high degree of temporal synchronization between the signal and idler photons. Through a numerical exercise, we find that the use of photonic crystal fiber (PCF) facilitates the fulfilment of the conditions for ultra-broadband photon pair generation; in particular, the spectral region in which emission occurs can be adjusted to particular needs through an appropriate choice of the PCF parameters. In addition, we present a novel quantum interference effect, resulting from indistinguishable pathways to the same outcome, which can occur when pumping a SFWM source with multiple spectral lines.