Abstract. Fires associated with land use and land cover changes release large amounts of aerosols and trace gases into the atmosphere. Although several inventories of biomass burning emissions cover Brazil, there are still considerable uncertainties and differences among them. While most fire emission inventories utilize the parameters of burned area, vegetation fuel load, emission factors, and other parameters to estimate the biomass burned and its associated emissions, several more recent inventories apply an alternative method based on fire radiative power (FRP) observations to estimate the amount of biomass burned and the corresponding emissions of trace gases and aerosols. The Brazilian Biomass Burning Emission Model (3BEM) and the Fire Inventory from NCAR (FINN) are examples of the first, while the Brazilian Biomass Burning Emission Model with FRP assimilation (3BEM_FRP) and the Global Fire Assimilation System (GFAS) are examples of the latter. These four biomass burning emission inventories were used during the South American Biomass Burning Analysis (SAMBBA) field campaign. This paper analyzes and inter-compared them, focusing on eight regions in Brazil and the time period of 1 September-31 October 2012. Aerosol optical thickness (AOT 550 nm ) derived from measurements made by the Moderate Resolution Imaging Spectroradiometer (MODIS) operating on board the Terra and Aqua satellites is also applied to assess the inventories' consistency. The daily area-averaged pyrogenic carbon monoxide (CO) emission estimates exhibit significant linear correlations (r, p > 0.05 level, Student t test) between 3BEM and FINN and between 3BEM_ FRP and GFAS, with values of 0.86 and 0.85, respectively. These results indicate that emission estimates in this region derived via similar methods tend to agree with one other. However, they differ more from the estimates derived via the alternative approach. The evaluation of MODIS AOT 550 nm indicates that model simulation driven by 3BEM and FINN typically underestimate the smoke particle loading in the eastern region of Amazon forest, while 3BEM_FRP estimations to the area tend to overestimate fire emissions. The daily regional CO emission fluxes from 3BEM and FINN have linear correlation coefficients of 0.75-0.92, with typically 20-30 % higher emission fluxes in FINN. The daily regional CO emission fluxes from 3BEM_FRP and GFAS show linear correlation coefficients between 0.82 and 0.90, with a particularly strong correlation near the arc of deforestation in the Amazon rainforest. In this region, GFAS has a tendency to present higher CO emissions than 3BEM_FRP, while 3BEM_FRP yields more emissions in the area of soybean expansion east of the Amazon forest. Atmospheric aerosol optical thickness is simulated by using the emission inventories with two operational atmospheric chemistry transport models: the Published by Copernicus Publications on behalf of the European Geosciences Union. However, the aerosol emissions from fires with particularly high biomass consumption still lead to ...
Abstract. We present a new version of the Brazilian developments on the Regional Atmospheric Modeling System (BRAMS), in which different previous versions for weather, chemistry, and carbon cycle were unified in a single integrated modeling system software. This new version also has a new set of state-of-the-art physical parameterizations and greater computational parallel and memory usage efficiency. The description of the main model features includes several examples illustrating the quality of the transport scheme for scalars, radiative fluxes on surface, and model simulation of rainfall systems over South America at different spatial resolutions using a scale aware convective parameterization. Additionally, the simulation of the diurnal cycle of the convection and carbon dioxide concentration over the Amazon Basin, as well as carbon dioxide fluxes from biogenic processes over a large portion of South America, are shown. Atmospheric chemistry examples show the model performance in simulating near-surface carbon monoxide and ozone in the Amazon Basin and the megacity of Rio de Janeiro. For tracer transport and dispersion, the model capabilities to simulate the volcanic ash 3-D redistribution associated with the eruption of a Chilean volcano are demonstrated. The gain of computational efficiency is described in some detail. BRAMS has been applied for research and operational forecasting mainly in South America. Model results from the operational weather forecast of BRAMS on 5 km grid spacing in the Center for Weather Forecasting and Climate Studies, INPE/Brazil, since 2013 are used to quantify the model skill of near-surface variables and rainfall. The scores show the reliability of BRAMS for the tropical and subtropical areas of South America. Requirements for keeping this modeling system competitive regarding both its functionalities and skills are discussed. Finally, we highlight the relevant contribution of this work to building a South American community of model developers.
<p><strong>Abstract.</strong> Fires associated with land use and land cover changes release into the atmosphere large amounts of aerosols and trace gases. Although there are several inventories of biomass burning emissions covering Brazil, there are still considerable uncertainties and differences among these. While most fire emissions inventories still utilize the parameters of vegetation fuel load, emission factors and other parameters to estimate the biomass burned and its associated emissions, certain more recent inventories tend to apply an alternative method based on fire radiative power (FRP) observations to estimate the amount of biomass burned and the corresponding emissions of trace gases and aerosols. The Brazilian Biomass Burning Emission Model (3BEM) and Fire Inventory from NCAR (FINN) are examples of the first, while Brazilian Biomass Burning Emission Model with FRP assimilation (3BEM_FRP) and Global Fire Assimilation System (GFAS) are examples of the latter method mentioned. In this paper, the output of four biomass burning emission inventories used during the South American Biomass Burning Analysis (SAMBBA) field campaign are analyzed and intercompared, focusing on eight predefined grids. Aerosol optical thickness derived from measurements made by the MODIS sensor operating onboard the Aqua satellite is applied to assess the inventories consistency. Significant correlation coefficients (r, p>0.05 level, Student t-test) were found between 3BEM and FINN, and between 3BEM_FRP and GFAS, with approximately 0.86 and 0.85, respectively. These results indicate that emissions estimates in this region derived via similar methods tend to agree with one other, but differ more from the estimates derived via the alternative approach. However, correlations in specific grids indicate that 3BEM and FINN typically underestimated the smoke emission loading in the eastern region of Amazon Forest, whilst 3BEM_FRP presents a tendency to overestimate fire emissions in the same area. The relationship between the 3BEM and FINN fire inventories present a correlation coefficient of 0.75-0.92, with a tendency of FINN to overestimate the emission of carbon monoxide by 20-30%. Moreover, 3BEM and GFAS shows a correlation coefficient of between 0.75-0.85, with higher values near the arc of deforestation in Amazon Rainforest. However, GFAS has a tendency to present higher carbon monoxide emissions in this region, and 3BEM_FRP tends to overestimate the emissions in soybean expansion (east of Amazon forest).</p>
Multifilter rotating shadowband radiometer (MFRSR) calibration values for aerosol optical depth (AOD) retrievals were determined by means of the general method formulated by Forgan [Appl. Opt.33, 4841 (1994)] at a polluted urban site. The obtained precision is comparable with the classical method, the Langley plot, applied on clean mountaintops distant of pollution sources. The AOD retrieved over São Paulo City with both calibration procedures is compared with the Aerosol Robotic Network data. The observed results are similar, and, except for the shortest wavelength (415 nm), the MFRSR's AOD is systematically overestimated by approximately 0.03.
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