Background: Few European studies have investigated the effects of long-term exposure to both fine particulate matter (≤ 2.5 µm; PM2.5) and nitrogen dioxide (NO2) on mortality.Objectives: We studied the association of exposure to NO2, PM2.5, and traffic indicators on cause-specific mortality to evaluate the form of the concentration–response relationship.Methods: We analyzed a population-based cohort enrolled at the 2001 Italian census with 9 years of follow-up. We selected all 1,265,058 subjects ≥ 30 years of age who had been living in Rome for at least 5 years at baseline. Residential exposures included annual NO2 (from a land use regression model) and annual PM2.5 (from a Eulerian dispersion model), as well as distance to roads with > 10,000 vehicles/day and traffic intensity. We used Cox regression models to estimate associations with cause-specific mortality adjusted for individual (sex, age, place of birth, residential history, marital status, education, occupation) and area (socioeconomic status, clustering) characteristics.Results: Long-term exposures to both NO2 and PM2.5 were associated with an increase in nonaccidental mortality [hazard ratio (HR) = 1.03 (95% CI: 1.02, 1.03) per 10-µg/m3 NO2; HR = 1.04 (95% CI: 1.03, 1.05) per 10-µg/m3 PM2.5]. The strongest association was found for ischemic heart diseases (IHD) [HR = 1.10 (95% CI: 1.06, 1.13) per 10-µg/m3 PM2.5], followed by cardiovascular diseases and lung cancer. The only association showing some deviation from linearity was that between NO2 and IHD. In a bi-pollutant model, the estimated effect of NO2 on mortality was independent of PM2.5.Conclusions: This large study strongly supports an effect of long-term exposure to NO2 and PM2.5 on mortality, especially from cardiovascular causes. The results are relevant for the next European policy decisions regarding air quality.
We found an association of the pollution sources with some cancer forms and cardio-respiratory diseases. Although there was a high correlation between the estimated exposures, an indication of specific effects from the different sources emerged.
Particulate matter mass concentrations measured in the city of Rome (Italy) in the period 2001–2004 have been cross-analysed with concurrent Saharan dust advection events to infer the impact these natural episodes bear on the standard air quality parameter PM10 observed at two city stations and at one regional background station. Natural events such as Saharan dust advections are associated with a definite health risk. At the same time, the Directive 2008/50/EC allows subtraction of PM exceedances caused by natural contributions from statistics used to determine air quality of EU sites. In this respect, it is important to detect and characterise such advections by means of reliable, operational techniques. To assess the PM10 increase we used both the "regional-background method" suggested by EC Guidelines and a "local background" method, demonstrated to be most suited to this central Mediterranean region. In terms of exceedances, the two approaches provided results within ~20% of each other at background sites, and at ~50% of each other in traffic conditions.
The sequence of Saharan advections over the city has been either detected by Polarization Lidar (laser radar) observations or forecast by the operational numerical regional mineral dust model BSC-DREAM8b of the Barcelona Supercomputing Centre. Lidar observations were also employed to retrieve the average physical properties of the dust clouds as a function of height. Over the four-year period, Lidar measurements (703 evenly distributed days) revealed Saharan plumes transits over Rome on 28.6% of the days, with minimum occurrence in wintertime. Dust was observed to reach the ground on 17.5% of the days totalling 88 episodes. Most (90%) of these advections lasted up to 5 days, averaging to ~3 days. Median time lag between advections was 7 days. Typical altitude range of the dust plumes was 0–6 km, with the centre of mass at ~3 km a.g.l. BSC-DREAM8b model simulations (1461 days) predicted Lidar detectable (532 nm extinction coefficient > 0.005 km−1) dust advections on 25.9% of the days, with ground contacts on 13% of the days. As in the Lidar case, the average dust centre of mass was forecast at ~3 km. Along the 703 day Lidar dataset, model forecast and Lidar detection of the presence of dust coincided on 80% of the cases, 92% coincidences are found within a ±1 day window.
Combination of the BSC-DREAM8b and Lidar records leads to about 21% of the days being affected by presence of Saharan dust at the ground. This combined dataset has been used to compute the increase in PM with respect to dust-unaffected previous days. This analysis has shown Saharan dust events to exert a meaningful impact on the PM10 records, causing average increases of the order of 11.9 μg m−3. Conversely, PM10 increases computed relying only on the Lidar detections (i.e., presence of dust layers actually observed) were of the order of 15.6 μg m−3. Both analyses indicate the annual average contrib...
An experimental campaign, Study of the Atmospheric Boundary Layer Environmental at Dome C, was held during 2005 at the French-Italian station of Concordia at Dome C. Ground-based remote sensors, as well as in situ instrumentation, were used during the experimental campaign. The measurements allowed the direct estimation of the polar atmospheric boundary-layer height and the test of several parametrizations for the unstable and stable boundary layers. During the months of January and February, weak convection was observed while, during the polar night, a long-lived stable boundary layer occurred continuously. Under unstable stratification the mixing-layer height was determined using the sodar backscattered echoes and potential temperature profiles. The two estimations are highly correlated, with the mixing height ranging between 30 and 350 m. A simple prognostic one-dimensional model was used to estimate the convective mixing-layer height, with the correlation coefficient between observations and model results being 0.66. The boundarylayer height under stable conditions was estimated from radiosounding profiles as the height where the critical Richardson number is reached; values between 10 and 150 m were found. A visual inspection of potential temperature profiles was also used as further confirmation of the experimental height; the results of the two methods are in good agreement. Six parametrizations from the literature for the stable boundary-layer height were tested. Only the parametrization that considers the long-lived stable boundary layer and takes into account the interaction of the stable layer with the free atmosphere is in agreement with the observations.
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