Superconductivity was recently observed in iron-arsenic-based compounds with a superconducting transition temperature (T(c)) as high as 56 K, naturally raising comparisons with the high-T(c) copper oxides. The copper oxides have layered crystal structures with quasi-two-dimensional electronic properties, which led to speculation that reduced dimensionality (that is, extreme anisotropy) is a necessary prerequisite for superconductivity at temperatures above 40 K (refs 8, 9). Early work on the iron-arsenic compounds seemed to support this view. Here we report measurements of the electrical resistivity in single crystals of (Ba,K)Fe(2)As(2) in a magnetic field up to 60 T. We find that the superconducting properties are in fact quite isotropic, being rather independent of the direction of the applied magnetic fields at low temperature. Such behaviour is strikingly different from all previously known layered superconductors, and indicates that reduced dimensionality in these compounds is not a prerequisite for 'high-temperature' superconductivity. We suggest that this situation arises because of the underlying electronic structure of the iron-arsenic compounds, which appears to be much more three dimensional than that of the copper oxides. Extrapolations of low-field single-crystal data incorrectly suggest a high anisotropy and a greatly exaggerated zero-temperature upper critical field.
Retaining a dissipation-free state while carrying large electrical currents is a challenge that needs to be solved to enable commercial applications of high-temperature superconductivity. Here, we show that the controlled combination of two effective pinning centres (randomly distributed nanoparticles and self-assembled columnar defects) is possible and effective. By simply changing the temperature or growth rate during pulsed-laser deposition of BaZrO(3)-doped YBa(2)Cu(3)O(7) films, we can vary the ratio of these defects, tuning the field and angular critical-current (Ic) performance to maximize Ic. We show that the defects' microstructure is governed by the growth kinetics and that the best results are obtained with a mixture of splayed columnar defects and random nanoparticles. The very high Ic arises from a complex vortex pinning landscape where columnar defects provide large pinning energy, while splay and nanoparticles inhibit flux creep. This knowledge is used to produce thick films with remarkable Ic(H) and nearly isotropic angle dependence.
We present resistivity measurements of the complete superconducting upper critical field (H{c2}) phase diagram as a function of angle (theta) and temperature (T) for cobalt-doped SrFe2As2 epitaxial films to 0.5 K and 50 T. Although H{c2}(theta) at 10 K is indistinguishable from that derived from a single-band anisotropy model, the apparent anisotropy H{c2}{ perpendicularc}/H{c2};{ parallelc} linearly decreases to 1 at low T, with H{c2}(0)=47 T. The data are well described by a two-band model with small, opposing anisotropies for the bands. This unusual relationship is confirmed by the observation of a local maximum for H{c2};{ parallelc} at low T.
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