Recordings of dynamic holograms with microsecond relaxation times under the action of nanosecond laser pulses are obtained in composites on the base of a novel class of liquid crystals (LCs) in ionic metal-alkanoates. Holographic parameters and relaxation characteristics are measured for doped lyotropic ionic LC, for sandwichlike cells (consisting of a dye layer and a layer of the lyotropic ionic LC), and for colored ionic smectic glasses. The structure of the materials is investigated by use of the small-angle x-ray technique. The mechanism of resonance nonlinearity in photosensitive centers and mechanisms of the grating erasure connected with a charge transport in the ionic conductive LC matrix are discussed.
The amplitude of the phase dynamic grating is a nonuniform space distributed in photorefractive crystals with nonlocal response as a result of energy transfer between the interacted waves. The dynamical process of grating formation in the case of transmission two- and four-wave mixing is described by the damped sine-Gordon equation that governs the soliton propagation. A stationary soliton solution for the grating amplitude profile was obtained. Experiments on observation of a nonuniform distribution of the grating amplitude through the crystal volume are presented. It is experimentally shown that the changes of the grating amplitude profile in dependence of input intensity ratio match the solutions of the damped sine-Gordon equation in steady state. The diffraction efficiency of energy transfer is determined by the value of the integral under the grating amplitude profile. The soliton profile is altered with changing input intensity ratio of recorded beams. It provides the effect of diffraction efficiency management by changing the half-width and the position of the soliton. The theory predicts a multisoliton behavior in reversible media with strong amplification gain that leads to auto-oscillations of output wave intensities.
We consider the dynamical degenerate four-wave mixing (FWM) model in a cubic nonlinear medium including both the time relaxation of the induced nonlinearity and the nonlocal coupling. The initial ten-dimensional FWM system can be rewritten as a three-variable intrinsic system (namely, the intensity pattern, the amplitude of the nonlinearity, and the total net gain) which is very close to the pumped Maxwell-Bloch system. In the case of a purely nonlocal response the initial system reduces to a real damped sine-Gordon (SG) equation. We obtain a solution of this equation in the form of a sech function with a time-dependent coefficient. By applying the reductive perturbation method to this damped SG equation, we obtain exactly the cubic complex Ginzburg Landau equation (CGL3) but with a time dependence in the loss or gain coefficient. The CGL3 describes the properties of the spatially localized interference pattern formed by the FWM.
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