An axion insulator is a correlated topological phase, predicted to arise from the formation of a charge density wave in a Weyl semimetal. The accompanying sliding mode in the charge density wave phase, the phason, is an axion. It is expected to cause anomalous magneto-electric transport effects. However, this axionic charge density wave has so far eluded experimental detection. In this paper, we report the observation of a large, positive contribution to the magneto-conductance in the sliding mode of the charge density wave Weyl semimetal (TaSe4)2I for collinear electric and magnetic fields (E||B).The positive contribution to the magneto-conductance originates from the anomalous axionic contribution of the chiral anomaly to the phason current, and is locked to the parallel alignment of E and B. By rotating B, we show that the angular dependence of the magneto-conductance is consistent with the anomalous transport of an axionic charge density wave. 3 Axions refer to elementary particles that have long been known in quantum field theory, 1,2 but have yet to be observed in nature. However, it has been recently understood that axions can emerge as collective electronic excitations in certain crystals, so-called axion insulators. 3 Despite being fully gapped to single-particle excitations in the bulk and at the surface, an axion insulator is characterized by an effective action, which includes a topological EB-term, where E and B are the electromagnetic fields inside the insulator, and plays the role of the dynamical axion field. Physically, the average value of is determined by the microscopic details of the band structure of the system, and gives rise to unusual magnetoelectric response properties such as quantum anomalous Hall conductivities 4-9 , the quantized circular photo-galvanic 4,10,11 effect, and the chiral magnetic effect. 4,[12][13][14] The prospect of realizing an axion insulator has inspired much theoretical and experimental work. Only very recently, signatures of a dynamic axion field have been found on the surface of magnetically doped topological insulator thin films. [15][16][17] However, the axionic quasi-particle in these systems-the axionic polariton 3 -has so far eluded experimental detection. Alternatively, axion insulators have been predicted to arise in Weyl semimetals that are unstable towards the formation of a charge density wave (CDW). [18][19][20][21][22][23] In their parent state, Weyl semimetals are materials in which the low-energy electronic quasiparticles behave as chiral relativistic fermions without rest mass, known as Weyl fermions. [24][25][26][27] The Weyl fermions exist at isolated crossing points of conductance and valence bands-so called Weyl nodes-and their energy can be approximated with a linear dispersion relation ( Fig. 1 (a)). The Weyl nodes always occur in pairs of opposite "handedness" or chirality. At low energies and in the absence of interactions the chirality is a conserved quantum number, and the two chiral populations do not mix. Parallel electric and mag...
Interacting electrons confined to their lowest Landau level in a high magnetic field can form a variety of correlated states, some of which manifest themselves in a Hall effect. Although such states have been predicted to occur in three-dimensional semimetals, a corresponding Hall response has not yet been experimentally observed. Here, we report the observation of an unconventional Hall response in the quantum limit of the bulk semimetal HfTe5, adjacent to the three-dimensional quantum Hall effect of a single electron band at low magnetic fields. The additional plateau-like feature in the Hall conductivity of the lowest Landau level is accompanied by a Shubnikov-de Haas minimum in the longitudinal electrical resistivity and its magnitude relates as 3/5 to the height of the last plateau of the three-dimensional quantum Hall effect. Our findings are consistent with strong electron-electron interactions, stabilizing an unconventional variant of the Hall effect in a three-dimensional material in the quantum limit.
The possibility of tuning magnetic material properties by ionic means is exciting both for basic science and, especially in view of the excellent energy efficiency and room temperature operation, for potential applications. In this perspective, we shortly introduce the functionality of magneto-ionic materials and focus on important recent advances in this field. We present a comparative overview of state-of-the-art magneto-ionic materials considering the achieved magnetoelectric voltage coefficients for magnetization and coercivity and the demonstrated time scales for magneto-ionic switching. Furthermore, the application perspectives of magneto-ionic materials in data storage and computing, magnetic actuation, and sensing are evaluated. Finally, we propose potential research directions to push this field forward and tackle the challenges related to future applications.
The perspective of energy-efficient and tunable functional magnetic nanostructures has triggered research efforts in the fields of voltage control of magnetism and spintronics. We investigate the magnetotransport properties of nanocomposite iron oxide/iron thin films with a nominal iron thickness of 5−50 nm and find a positive magnetoresistance at small thicknesses. The highest magnetoresistance was found for 30 nm Fe with +1.1% at 3 T. This anomalous behavior is attributed to the presence of Fe 3 O 4 −Fe nanocomposite regions due to grain boundary oxidation. At the Fe 3 O 4 /Fe interfaces, spin-polarized electrons in the magnetite can be scattered and reoriented. A crossover to negative magnetoresistance (−0.11%) is achieved at a larger thickness (>40 nm) when interface scattering effects become negligible as more current flows through the iron layer. Electrolytic gating of this system induces voltage-triggered redox reactions in the Fe 3 O 4 regions and thereby enables voltage-tuning of the magnetoresistance with the locally oxidized regions as the active tuning elements. In the low-magnetic-field region (<1 T), a crossover from positive to negative magnetoresistance is achieved by a voltage change of only 1.72 V. At 3 T, a relative change of magnetoresistance about −45% during reduction was achieved for the 30 nm Fe sample. The present low-voltage approach signifies a step forward to practical and tunable room-temperature magnetoresistance-based nanodevices, which can boost the development of nanoscale and energy-efficient magnetic field sensors with high sensitivity, magnetic memories, and magnetoelectric devices in general.
A comparative study of the anodization processes occurring at the GaAs(111)A and GaAs(111)B surfaces exposed to electrochemical etching in neutral NaCl and acidic HNO3 aqueous electrolytes is performed in galvanostatic and potentiostatic anodization modes. Anodization in NaCl electrolytes was found to result in the formation of porous structures with porosity controlled either by current under the galvanostatic anodization, or by the potential under the potentiostatic anodization. Possibilities to produce multilayer porous structures are demonstrated. At the same time, one-step anodization in a HNO3 electrolyte is shown to lead to the formation of GaAs triangular shape nanowires with high aspect ratio (400 nm in diameter and 100 µm in length). The new data are compared to those previously obtained through anodizing GaAs(100) wafers in alkaline KOH electrolyte. An IR photodetector based on the GaAs nanowires is demonstrated.
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