The advanced molybdenum-based rare process experiment (AMoRE) aims to search for neutrinoless double beta decay ($$0\nu \beta \beta $$0νββ) of $$^{100}$$100Mo with $$\sim 100\,\hbox {kg}$$∼100kg of $$^{100}$$100Mo-enriched molybdenum embedded in cryogenic detectors with a dual heat and light readout. At the current, pilot stage of the AMoRE project we employ six calcium molybdate crystals with a total mass of 1.9 kg, produced from $$^{48}$$48Ca-depleted calcium and $$^{100}$$100Mo-enriched molybdenum ($$^{48{{\text {depl}}}}\hbox {Ca}^{100}\hbox {MoO}_{4}$$48deplCa100MoO4). The simultaneous detection of heat (phonon) and scintillation (photon) signals is realized with high resolution metallic magnetic calorimeter sensors that operate at milli-Kelvin temperatures. This stage of the project is carried out in the Yangyang underground laboratory at a depth of 700 m. We report first results from the AMoRE-Pilot $$0\nu \beta \beta $$0νββ search with a 111 kg day live exposure of $$^{48{{\text {depl}}}}\hbox {Ca}^{100}\hbox {MoO}_{4}$$48deplCa100MoO4 crystals. No evidence for $$0\nu \beta \beta $$0νββ decay of $$^{100}$$100Mo is found, and a upper limit is set for the half-life of $$0\nu \beta \beta $$0νββ of $$^{100}$$100Mo of $$T^{0\nu }_{1/2} > 9.5\times 10^{22}~\hbox {years}$$T1/20ν>9.5×1022years at 90% C.L. This limit corresponds to an effective Majorana neutrino mass limit in the range $$\langle m_{\beta \beta }\rangle \le (1.2-2.1)\,\hbox {eV}$$⟨mββ⟩≤(1.2-2.1)eV.
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The AMoRE (Advanced Mo-based Rare process Experiment) project is a series of experiments that use advanced cryogenic techniques to search for the neutrinoless double-beta decay of 100 Mo. The work is being carried out by an international collaboration of researchers from eight countries. These searches involve high precision measurements of radiation-induced temperature changes and scintillation light produced in ultra-pure 100 Mo-enriched and 48 Ca-depleted calcium molybdate ( 48depl Ca 100 MoO 4 ) crystals that are located in a deep underground laboratory in Korea. The 100 Mo nuclide was chosen for this 0νββ decay search because of its high Q-value and favorable nuclear matrix element. Tests have demonstrated that CaMoO 4 crystals produce the brightest scintillation light among all of the molybdate crystals, both at room and at cryogenic temperatures. 48depl Ca 100 MoO 4 crystals are being operated at milli-Kelvin temperatures and read out via specially developed metallic-magnetic-calorimeter (MMC) temperature sensors that have excellent energy resolution and relatively fast response times. The excellent energy resolution provides good discrimination of signal from backgrounds, and the fast response time is important for minimizing the irreducible background caused by random coincidence of two-neutrino double-beta decay events of 100 Mo nuclei. Comparisons of the scintillating-light and phonon yields and pulse shape discrimination of the phonon signals will be used to provide redundant rejection of alpha-ray-induced backgrounds. An effective Majorana neutrino mass sensitivity that reaches the expected range of the inverted neutrino mass hierarchy, i.e., 20-50 meV, could be achieved with a 200 kg array of 48depl Ca 100 MoO 4 crystals operating for three years.
Background: A double K-electron capture is a rare nuclear-atomic process in which two K electrons are captured simultaneously from the atomic shell. A "hollow atom" is created as a result of this process. In single K shell electron-capture decays, there is a small probability that the second electron in the K-shell is excited to an unoccupied level or can (mostly) be ejected to the continuum. In either case, a double vacancy is created in the K-shell. The relaxation of the double K-shell vacancy, accompanied by the emission of two K-fluorescence photons, makes it possible to perform experimental studies of such rare processes with the large-volume proportional gas chamber. Purpose: The purpose of the present analysis is to estimate a double-K-shell vacancy creation probability per K-shell electron capture PKK of 81 Kr, as well as to measure the half-life of 78 Kr relative to 2ν2K capture. Method: Time-resolving current pulse from the large low-background proportional counter (LPC), filled with the krypton sample, was applied to detect triple coincidences of "shaked" electrons and two fluorescence photons. Results: The number of K-shell vacancies per the K-electron capture, produced as a result of the shake-off process, has been measured for the decay of 81 Kr. The probability for this decay was found to be PKK = (5.7 ± 0.8) × 10 −5 with a systematic error of (∆PKK )syst = ±0.4 × 10 −5 . For the 78 Kr(2ν2K) decay, the comparative study of single-and double-capture decays allowed us to obtain the signal-to-background ratio up to 15/1. The half-life22 y is determined from the analysis of data that have been accumulated over 782 days of live measurements in the experiment that used samples consisted of 170.6 g of 78 Kr. Conclusions: The data collected during low background measurements using the LPC were analyzed to search the rare atomic and nuclear processes. We have determined P exp KK for the EC decay of 81 Kr, which are in satisfactory agreement with Z −2 dependence of PKK predicted by Primakoff and Porter. This made possible to more accurately determine the background contribution in the energy region of our interest for the search for the 2K-capture in 78 Kr. The general procedure of data analysis allowed us to determine the half-life of 78 Kr relative to 2ν2K-transition with a greater statistical accuracy than in our previous works.
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