We
demonstrate the use of ball milling mechanochemistry for rapid,
simple, and materials-efficient synthesis of the organic mineral paceite
CaCu(OAc)
4
·6H
2
O (where OAc
–
is the acetate ion), composed of coordination polymer chains containing
alternating Ca
2+
and Cu
2+
ions, as well as its
cadmium-based analogue CaCd(OAc)
4
·6H
2
O.
While the synthesis of paceite in aqueous solutions requires a high
excess of the copper precursor, mechanochemistry permits the use of
stoichiometric amounts of reagents, as well as the use of poorly soluble
and readily accessible calcium carbonate or hydroxide reactants. As
established by thermochemical measurements, enthalpies of formation
of both synthetic paceite and its cadmium analogue relevant to the
mechanochemical reactions are highly exothermic. Reactions can also
be conducted using accelerated aging, a synthetic technique that mimics
geological processes of mineral weathering. Accelerated aging reactivity
involving copper(II) acetate monohydrate (hoganite) and calcium carbonate
(calcite) provides a potential explanation of how complex organic
minerals like paceite could form in a geological environment.
Artificial intelligence has developed rapidly in recent years. Deep neural networks are the basis of many artificial intelligence applications. How to accelerate the computational processing of deep neural networks is very important. To explor the potential for accelerating the process deep neural networks on various hardware platforms, we propose a convolutional neural network optimization method based on the Weight-Stationary for SW26010 processor. We re-circulate convolution loops and use hybrid DMA transmission mode to increase memory bandwidth and reduce memory access overhead. On top of those, further optimizations are done based on register communication, asynchronous DMA transfer double buffering, instruction scheduling and other schemes. Finally, we achieve a double-precision convolution performance over 2.4 Tflops, achieving 81% of the processor's peak performance. In multiple parameters, we achieve a proforamnce acceleration of 2.4 − 4.0× speedup compared to the Tesla K80 GPU with cuDNNv7.
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