Intrinsically stretchable electronics represent an attractive platform for next-generation implantable devices by reducing the mechanical mismatch and the immune responses with biological tissues. Despite extensive efforts, soft implantable electronic devices often exhibit an obvious trade-off between electronic performances and mechanical deformability because of limitations of commonly used compliant electronic materials. Here, we introduce a scalable approach to create intrinsically stretchable and implantable electronic devices featuring the deployment of liquid metal components for ultrahigh stretchability up to 400% tensile strain and excellent durability against repetitive deformations. The device architecture further shows long-term stability under physiological conditions, conformal attachments to internal organs, and low interfacial impedance. Successful electrophysiological mapping on rapidly beating hearts demonstrates the potential of intrinsically stretchable electronics for widespread applications in health monitoring, disease diagnosis, and medical therapies.
Stretchable alternating current electroluminescent display is an emerging form of light-emitting device by combining elasticity with optoelectronic properties. The practical implementations are currently impeded by the high operating voltages required to achieve sufficient brightness. In this study, we report the development of dielectric nanocomposites by filling surface-modified ceramic nanoparticles into polar elastomers, which exhibit a series of desirable attributes, in terms of high permittivity, mechanical deformability, and solution processability. Dielectric nanocomposite effectively concentrates electric fields onto phosphor to enable low-voltage operation of stretchable electroluminescent display, thereby alleviating safety concerns toward wearable applications. The practical feasibility is demonstrated by an epidermal stopwatch that allows intimate integration with the human body. The high-permittivity nanocomposites reported here represent an attractive building block for stretchable electronic systems, which may find broad range of applications in intrinsically stretchable transistors, sensors, light-emitting devices, and energy-harvesting devices.
Stretchable electroluminescent device is a compliant form of light-emitting device to expand the application areas of conventional optoelectronics on rigid wafers. Currently, practical implementations are impeded by the high operating voltage required to achieve sufficient brightness. In this study, we report the fabrication of an intrinsically stretchable electroluminescent device based on silver nanowire electrodes and high-k thermoplastic elastomers. The device exhibits a bright emission with a low driving voltage by using polar elastomer as a dielectric matrix of the electroluminescent layer. Highly stretchable silver nanowire electrodes contribute to the exceptional elasticity and durability of the device in spite of bending, stretching, twisting, puncturing, and cutting. Stretchable electroluminescent devices developed here may find potential uses in wearable displays, deformable lightings, and soft robotics.
The rapid expansion of electronic technology and short lifespan of consumer devices create a huge amount of electronic waste. The disposal of discarded devices represents a serious environmental challenge. Biodegradable devices are able to decompose into benign components after a period of stable operation during its service life, which represents a potential solution to reduce the environmental footprint of electronic technology. The widespread applications of biodegradable electronics are still hampered by the lack of facile manufacturing approach for high quality devices. Here, a laser sintering technique to weld naturally oxidized Zn microparticles into biodegradable conductors is reported. The sintering process is carried out under ambient conditions and compatible with various biodegradable substrates. A low‐cost fabrication procedure involving stencil printing and laser treatment is established to create conductive features with excellent conductivity and mechanical durability. The practical suitability of printed Zn conductor is demonstrated by fabricating near‐field communication tags, which are flexible and fully functional with the transient behavior modulated by the choice of packaging materials. The printed biodegradable conductor may find potential applications in eco‐friendly sensors, transient printed circuit boards, and implantable medical devices.
Electronic textiles offer exciting opportunities for an emerging class of electronic technology featuring intimate interaction with the human body. Among various functional components, a stretchable conductive textile represents a key building material to support the development of sensors, interconnects, and electrical contacts. In this study, a conductive textile is synthesized by bottom-up coassembly of silver nanowires and TPU microfibers. The conformal coverage of AgNW network over individual TPU microfibers gives rise to coherent deformations to mitigate the actual strain for enhanced stretchability and durability. The as-prepared conductive microtextile exhibits a series of desirable properties including excellent conductivity (>5000 S cm–1), exceptional stretchability (∼600% strain), soft mechanical properties, breathability, and washability. The practical implementation is demonstrated by fabricating an integrated epidermal sensing sleeve for multichannel EMG signal recordings, which supports real-time hand gesture recognitions powered by machine learning algorithm as a smart human–machine interface. The conductive textile reported in this study is well suited for garment integrated electronics with potential applications in health monitoring, robotic prosthetics, and competitive sports.
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