Metamaterials, as artificially structured materials composed of subwavelength arrays of resonant unit cells, can exhibit exotic properties beyond those accessible to natural materials. They were initially proposed for challenging fundamental laws and demonstrating negative refraction in the microwave regime, and subsequently exploited as a versatile platform to manipulate electromagnetic waves throughout the spectrum via their extreme scalability. Over the past decade, research into metamaterials has been extended to a search for real-world applications, leading to the concept of metadevices, defined as metamaterial-based devices that can operate in an active manner. Due to their subwavelength scale, metamaterials present intriguing strategies for active tuning and provide flat, high-efficiency alternatives to conventional optical systems based on bulky components. In this topical review, we summarize the development of active metamaterials and metadevices ranging from microwave to visible wavelengths, including milestones as well as the state of the art. We survey tuning strategies based on mechanical reconfiguration and incorporation with active materials such as varactor diodes, semiconductors, liquid crystals, phase change materials, superconductors, and two-dimensional materials under various external stimuli, and discuss their fascinating advantages and potential challenges to be confronted. Finally, future prospects together with several emerging tuning strategies and materials are presented at the end.

Metamaterial analogues of electromagnetically induced transparency (EIT) have been intensively studied and widely employed for slow light and enhanced nonlinear effects. In particular, the active modulation of the EIT analogue and well-controlled group delay in metamaterials have shown great prospects in optical communication networks. Previous studies have focused on the optical control of the EIT analogue by integrating the photoactive materials into the unit cell, however, the response time is limited by the recovery time of the excited carriers in these bulk materials. Graphene has recently emerged as an exceptional optoelectronic material. It shows an ultrafast relaxation time on the order of picosecond and its conductivity can be tuned via manipulating the Fermi energy. Here we integrate a monolayer graphene into metal-based terahertz (THz) metamaterials, and realize a complete modulation in the resonance strength of the EIT analogue at the accessible Fermi energy. The physical mechanism lies in the active tuning the damping rate of the dark mode resonator through the recombination effect of the conductive graphene. Note that the monolayer morphology in our work is easier to fabricate and manipulate than isolated fashion. This work presents a novel modulation strategy of the EIT analogue in the hybrid metamaterials, and pave the way towards designing very compact slow light devices to meet future demand of ultrafast optical signal processing.

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Surface plasmon resonance (SPR) has been intensively studied and widely employed for light trapping and absorption enhancement. In the mid-infrared and terahertz (THz) regime, graphene supports tunable SPR via manipulating its Fermi energy and enhances light-matter interaction at the selected wavelength. Most previous studies have concentrated on the absorption enhancement in graphene itself while little attention has been paid to trapping light and enhancing the light absorption in other light-absorbing materials with graphene SPR. In this work, periodic arrays of graphene rings are proposed to introduce tunable light trapping with good angle polarization tolerance and enhance the absorption in the surrounding light-absorbing materials by more than one order of magnitude. Moreover, the design principle here could be set as a template to achieve multi-band plasmonic absorption enhancement by introducing more graphene concentric rings into each unit cell. This work not only opens up new ways of employing graphene SPR, but also leads to practical applications in high-performance simultaneous multi-color photodetection with high efficiency and tunable spectral selectivity.