In this study, we report a novel route via microwave irradiation to synthesize a bio-inspired hierarchical graphene--nanotube--iron three-dimensional nanostructure as an anode material in lithium-ion batteries. The nanostructure comprises vertically aligned carbon nanotubes grown directly on graphene sheets along with shorter branches of carbon nanotubes stemming out from both the graphene sheets and the vertically aligned carbon nanotubes. This bio-inspired hierarchical structure provides a three-dimensional conductive network for efficient charge-transfer and prevents the agglomeration and restacking of the graphene sheets enabling Li-ions to have greater access to the electrode material. In addition, functional iron-oxide nanoparticles decorated within the three-dimensional hierarchical structure provides outstanding lithium storage characteristics, resulting in very high specific capacities. The anode material delivers a reversible capacity of ~1024 mA · h · g(-1) even after prolonged cycling along with a Coulombic efficiency in excess of 99%, which reflects the ability of the hierarchical network to prevent agglomeration of the iron-oxide nanoparticles.
A simple strategy for the rapid preparation of multifunctional polydopamine (pDA) coatings is demonstrated. Microwave irradiation of the coating solution enables the formation of a ≈18 nm thick, genuine pDA coating in 15 min, which is ≈18 times faster than conventional coating. The acceleration effect results from the radical generation and temperature increase, which facilitate thermally accelerated radical polymerization of dopamine.
One of the most popular technologies in Web2.0 is tagging, and it widely applies to Web content as well as multimedia data such as image and video. Web users have expected that tags by themselves would be reused in information search and maximize the search efficiency, but wrong tag by irresponsible Web users really has brought forth a incorrect search results. In past papers, we have gathered various information resources and tags scattered in Web, mapped one tag onto other tags, and clustered these tags according to the corelation between them. A 3-tag based search algorithm which use the clustered tags of past papers, is proposed in this paper. For performance evaluation of the proposed algorithm, our algorithm is compared with image search result of Flickr, typical tag based site, and is evaluated in accuracy and recall factor.
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