Neutron diffraction measurements are presented exploring the magnetic and structural phase behaviors of the candidate J ef f = 1/2 Mott insulating iridate Sr2IrO4. Comparisons are drawn between the correlated magnetism in this single layer system and its bilayer analog Sr3Ir2O7 where both materials exhibit magnetic domains originating from crystallographic twinning and comparable moment sizes. Weakly temperature dependent superlattice peaks violating the reported tetragonal space group of Sr2IrO4 are observed supporting the notion of a lower structural symmetry arising from a high temperature lattice distortion, and we use this to argue that moments orient along a unique in-plane axis demonstrating an orthorhombic symmetry in the resulting spin structure. Our results demonstrate that the correlated spin order and structural phase behaviors in both single and bilayer Srn+1IrnO3n+1 systems are remarkably similar and suggest comparable correlation strengths in each system.
The Ruddlesden-Popper series of iridates (Srn+1IrnO3n+1) have been the subject of much recent attention due to the anticipation of emergent phenomena arising from the cooperative action of spin-orbit-driven band splitting and Coulomb interactions. However, an ongoing debate over the role of correlations in the formation of the charge gap and a lack of understanding of the effects of doping on the low-energy electronic structure have hindered experimental progress in realizing many of the predicted states. Using scanning tunnelling spectroscopy we map out the spatially resolved density of states in Sr3Ir2O7 (Ir327). We show that its parent compound, argued to exist only as a weakly correlated band insulator, in fact possesses a substantial ~ 130 meV charge excitation gap driven by an interplay between structure, spin-orbit coupling and correlations. We find that single-atom defects are associated with a strong electronic inhomogeneity, creating an important distinction between the intrinsic and spatially averaged electronic structure. Combined with first-principles calculations, our measurements reveal how defects at specific atomic sites transfer spectral weight from higher energies to the gap energies, providing a possible route to obtaining metallic electronic states from the parent insulating states in the iridates.
Through a neutron scattering, charge transport, and magnetization study, the correlated ground state in the bilayer iridium oxide Sr3Ir2O7 is explored. Our combined results resolve scattering consistent with a high temperature magnetic phase that persists above 600 K, reorients at the previously defined TAF = 280 K, and coexists with an electronic ground state whose phase behavior suggests the formation of a fluctuating charge or orbital phase that freezes below T * ≈ 70 K.Our study provides a window into the emergence of multiple electronic order parameters near the boundary of the metal to insulator phase transition of the 5d J ef f = 1/2 Mott phase.
The zonal electric field and the meridional neutral wind are the principal drivers that define the geometry and characteristics of the equatorial ionization anomaly (EIA). Here we present the response of the EIA to the variability of the zonal electric field based on measurements of the equatorial electrojet (EEJ) currents and trans‐equatorial neutral winds for the generation and control of the asymmetries of the EIA crests of total electron content (TEC) in the western side of the South American continent. The EEJ strengths are determined using a pair of magnetometers. The 24‐hr trans‐equatorial neutral wind profile is measured using the Second‐Generation, Optimized, Fabry‐Perot Doppler Imager (SOFDI) located near the geomagnetic equator. The EIA is evaluated using TEC data measured by Global Positioning System (GPS) receivers from the Low‐Latitude Ionospheric Sensor Network and several other networks in South America. A physics‐based numerical model, Low‐Latitude Ionospheric Sector, and SOFDI data are used to study the effects of daytime meridional neutral winds on the consequent evolution of an asymmetry in equatorial TEC anomalies during the afternoon and onward for the first time. We find that the configuration parameters such as strength, shape, amplitude, and latitudinal width of the EIAs are affected by the eastward electric field associated with the EEJ under undisturbed conditions. The asymmetries of EIA crests are observed more frequently during solstices and the September equinox than in the March equinox season. Importantly, this study indicates that the meridional neutral wind plays a very significant role in the development of the EIA asymmetry by transporting the plasma up the field lines. This result suggests that a precise observation of the latitudinal TEC profile at low latitudes can be used to derive the meridional wind.
This paper presents the interrelationship between the equatorial electrojet (EEJ) strength, Global Positioning System (GPS)‐derived total electron content (TEC), and postsunset scintillation from ground observations with the aim of finding reliable precursors of the occurrence of ionospheric irregularities. Mutual relationship studies provide a possible route to predict the occurrence of TEC fluctuation and scintillation in the ionosphere during the late afternoon and night respectively based on daytime measurement of the equatorial ionosphere. Data from ground based observations in the low latitudes of the west American longitude sector were examined during the 2008 solar minimum. We find a strong relationship exists between the noontime equatorial electrojet and GPS‐derived TEC distributions during the afternoon mediated by vertical E × B drift via the fountain effect, but there is little or no relationship with postsunset ionospheric scintillation.
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