Abstract. We have performed backward trajectory calculations and simulations with the three-dimensional Chemical Lagrangian Model of the Stratosphere (CLaMS) for two succeeding monsoon seasons using artificial tracers of air mass origin. With these tracers we trace back the origin of young air masses (age <6 months) at the top of the Asian monsoon anticyclone and of air masses within the tropical pipe (6 months < age <18 months) during summer 2008. The occurrence of young air masses (<6 months) at the top of the Asian monsoon anticyclone up to ∼460 K is in agreement with satellite measurements of chlorodifluoromethane (HCFC-22) by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) instrument. HCFC-22 can be considered as a regional tracer for continental eastern Asia and the Middle East as it is mainly emitted in this region. Our findings show that the transport of air masses from boundary layer sources in the region of the Asian monsoon into the tropical pipe occurs in three distinct steps. First, very fast uplift in “a convective range” transports air masses up to 360 K potential temperature within a few days. Second, air masses are uplifted from about 360 K up to 460 K within “an upward spiralling range” within a few months. The large-scale upward spiral extends from northern Africa to the western Pacific. The air masses are transported upwards by diabatic heating with a rate of up to 1–1.5 K per day, implying strong vertical transport above the Asian monsoon anticyclone. Third, transport of air masses occurs within the tropical pipe up to 550 K associated with the large-scale Brewer–Dobson circulation within ∼1 year. In the upward spiralling range, air masses are uplifted by diabatic heating across the (lapse rate) tropopause, which does not act as a transport barrier, in contrast to the extratropical tropopause. Further, in the upward spiralling range air masses from inside the Asian monsoon anticyclone are mixed with air masses convectively uplifted outside the core of the Asian monsoon anticyclone in the tropical adjacent regions. Moreover, the vertical transport of air masses from the Asian monsoon anticyclone into the tropical pipe is weak in terms of transported air masses compared to the transport from the monsoon anticyclone into the northern extratropical lower stratosphere. Air masses from the Asian monsoon anticyclone (India/China) contribute a minor fraction to the composition of air within the tropical pipe at 550 K (6 %), and the major fractions are from Southeast Asia (16 %) and the tropical Pacific (15 %).

Abstract. The Asian summer monsoon anticyclone (ASMA) is a major meteorological system of the upper troposphere–lower stratosphere (UTLS) during boreal summer. It is known to contain enhanced tropospheric trace gases and aerosols, due to rapid lifting from the boundary layer by deep convection and subsequent horizontal confinement. Given its dynamical structure, the ASMA represents an efficient pathway for the transport of pollutants to the global stratosphere. A detailed understanding of the thermal structure and processes in the ASMA requires accurate in situ measurements. Within the StratoClim project we performed state-of-the-art balloon-borne measurements of temperature, water vapor, ozone and aerosol backscatter from two stations on the southern slopes of the Himalayas. In total, 63 balloon soundings were conducted during two extensive monsoon-season campaigns, in August 2016 in Nainital, India (29.4∘ N, 79.5∘ E), and in July–August 2017 in Dhulikhel, Nepal (27.6∘ N, 85.5∘ E); one shorter post-monsoon campaign was also carried out in November 2016 in Nainital. These measurements provide unprecedented insights into the UTLS thermal structure, the vertical distributions of water vapor, ozone and aerosols, cirrus cloud properties and interannual variability in the ASMA. Here we provide an overview of all of the data collected during the three campaign periods, with focus on the UTLS region and the monsoon season. We analyze the vertical structure of the ASMA in terms of significant levels and layers, identified from the temperature and potential temperature lapse rates and Lagrangian backward trajectories, which provides a framework for relating the measurements to local thermodynamic properties and the large-scale anticyclonic flow. Both the monsoon-season campaigns show evidence of deep convection and confinement extending up to 1.5–2 km above the cold-point tropopause (CPT), yielding a body of air with high water vapor and low ozone which is prone to being lifted further and mixed into the free stratosphere. Enhanced aerosol backscatter also reveals the signature of the Asian tropopause aerosol layer (ATAL) over the same region of altitudes. The Dhulikhel 2017 campaign was characterized by a 5 K colder CPT on average than in Nainital 2016 and a local water vapor maximum in the confined lower stratosphere, about 1 km above the CPT. Data assessment and modeling studies are currently ongoing with the aim of fully exploring this dataset and its implications with respect to stratospheric moistening via the ASMA system and related processes.

&lt;p&gt;&lt;strong&gt;Abstract.&lt;/strong&gt; The Asian summer monsoon anticyclone (ASMA) is a major meteorological system of the upper troposphere-lower stratosphere (UTLS) during boreal summer. It is known to be enriched in tropospheric trace gases and aerosols, due to rapid lifting from the boundary layer by deep convection and subsequent horizontal confinement. Given its dynamical structure, the ASMA offers a very efficient pathway for the transport of pollutants to the global stratosphere. Detailed understanding of the ASMA structure and processes requires accurate in-situ measurements. Here we present balloon-borne measurements of temperature, water vapor, ozone and aerosol backscatter conducted within the StratoClim project from two stations at the southern slopes of the Himalayas. In total we performed 63 balloon soundings during two main monsoon-season campaigns, in August 2016 in Nainital, India (NT16AUG) and July&amp;#8211;August 2017 in Dhulikhel, Nepal (DK17), and one brief post-monsoon campaign in Nainital in November 2016 (NT16NOV). These measurements provide unprecedented insights into the ASMA thermal structure and its relations to the vertical distributions of water vapor, ozone and aerosols. To study the structure of the UTLS during the monsoon season, we adopt the thermal definition of tropical tropopause layer (TTL), and define the region of altitudes between the lapse rate minimum (LRM) and the cold-point tropopause (CPT) as the Asian Tropopause Transition Layer (ATTL). Further, based on air mass trajectories, we define the Top of Confinement (TOC) level of ASMA, which divides the lower stratosphere (LS) into a Confined LS (CLS), below the TOC and above the CPT, and a Free LS (FLS), above the TOC. Using these thermodynamically-significant boundaries, our analysis reveals that the composition of the UTLS is affected by deep convection up to altitudes 1.5&amp;#8211;2&amp;#8201;km above the CPT due to the horizontal confinement effect of ASMA. This is shown by enhanced water vapor mixing ratios in the Confined LS compared to background stratospheric values in the Free LS, observed in both NT16AUG (+0.5&amp;#8201;ppmv) and DK17 (+0.75&amp;#8201;ppmv), and by enhanced aerosol backscatter of the Asian tropopause aerosol layer (ATAL) extending into the Confined LS, as observed in NT16AUG. The CPT was 600&amp;#8201;m higher in altitude and 5&amp;#8201;K colder in DK17 compared to NT16AUG and strong ozone depletion was found in the ATTL and CLS in DK17, suggesting stronger convective activity during DK17 compared to NT16AUG. An isolated water vapor maximum in the Confined LS, about 1&amp;#8201;km above the CPT, was also found in DK17, which we argue is due to overshooting convection hydrating the CLS. These evidence show that the vertical distributions and variability of water vapor, ozone and aerosols in the Asian UTLS are controlled by the top height of the anticyclonic confinement in ASMA, rather than by CPT height as in the conventional understanding of TTL, and suggest that the ASMA contributes to moistening the global stratosphere and to increase its aerosol burden.&lt;/p&gt;

Abstract. The South Asian summer monsoon is associated with a large-scale anticyclonic circulation in the upper troposphere and lower stratosphere (UTLS), which confines the air mass inside. During boreal summer, the confinement of this air mass leads to an accumulation of aerosol between about 13 and 18 km (360 and 440 K potential temperature); this accumulation of aerosol constitutes the Asian Tropopause Aerosol Layer (ATAL). We present balloon-borne aerosol backscatter measurements of the ATAL performed by the Compact Optical Backscatter Aerosol Detector (COBALD) instrument in Nainital in northern India in August 2016, and compare these with COBALD measurements in the post-monsoon time in November 2016. The measurements demonstrate a strong variability of the ATAL's altitude, vertical extent, aerosol backscatter intensity and cirrus cloud occurrence frequency. Such a variability cannot be deduced from climatological means of the ATAL as they are derived from satellite measurements. To explain this observed variability we performed a Lagrangian back-trajectory analysis using the Chemical Lagrangian Model of the Stratosphere (CLaMS). We identify the transport pathways as well as the source regions of air parcels contributing to the ATAL over Nainital in August 2016. Our analysis reveals a variety of factors contributing to the observed day-to-day variability of the ATAL: continental convection, tropical cyclones (maritime convection), dynamics of the anticyclone and stratospheric intrusions. Thus, the air in the ATAL is a mixture of air masses coming from different atmospheric altitude layers. In addition, contributions from the model boundary layer originate in different geographic source regions. The location of the strongest updraft along the backward trajectories reveals a cluster of strong upward transport at the southern edge of the Himalayan foothills. From the top of the convective outflow level (about 13 km; 360 K) the air parcels ascend slowly to ATAL altitudes within a large-scale upward spiral driven by the diabatic heating in the anticyclonic flow of the South Asian summer monsoon at UTLS altitudes. Cases with a strong ATAL typically show boundary layer contributions from the Tibetan Plateau, the foothills of the Himalayas and other continental regions below the Asian monsoon. Weaker ATAL cases show higher contributions from the maritime boundary layer, often related to tropical cyclones, indicating a mixing of clean maritime and polluted continental air. On the one hand increasing anthropogenic emissions in the future are expected due to the strong growth of Asian economies; on the other hand the implementation of new emission control measures (in particular in China) has reduced the anthropogenic emissions of some pollutants contributing to the ATAL substantially. It needs to be monitored in the future whether the thickness and intensity of the ATAL will further increase, which will likely impact the surface climate.