In this work we report on inelastic X-ray scattering experiments combined with the molecular dynamics simulations on deeply supercritical Ar. The presented results unveil the mechanism and regimes of sound propagation in the liquid matter, and provide a compelling evidence for the adiabatic-to-isothermal longitudinal sound propagation transition. We introduce a Hamiltonian predicting low-frequency transverse sound propagation gaps which is confirmed by experimental findings and molecular dynamics calculations. As a result, a universal link is established between the positive sound dispersion (PSD) phenomenon and the origin of transverse sound propagation revealing the viscous-to-elastic crossover in liquids. The PSD and transverse phononic excitations evolve consistently with theoretical predictions. Both can be considered as a universal fingerprint of the dynamic response of a liquid which is also observable in a sub-domain of supercritical phase. The simultaneous disappearance of both these effects at elevated temperatures is a manifestation of the Frenkel line. We expect that these findings will advance the current understanding of fluids under extreme thermodynamic conditions.
Owing to the depth to which hard X-rays penetrate into most materials, it is commonly accepted that the only way to realize hard-X-ray mirrors with near 100% reflectance is under conditions of total external reflection at grazing incidence to a surface. At angles away from grazing incidence, substantial reflectance of hard X-rays occurs only as a result of constructive interference of the waves scattered from periodically ordered atomic planes in crystals (Bragg diffraction). Theory predicts that even at normal incidence the reflection of X-rays from diamond under the Bragg condition should approach 100%-substantially higher than from any other crystal. Here we demonstrate that commercially produced synthetic diamond crystals do indeed show an unprecedented reflecting power at normal incidence and millielectronvolt-narrow reflection bandwidths for hard X-rays. Bragg diffraction measurements of reflectivity and the energy bandwidth show remarkable agreement with theory. Such properties are valuable to the development of hard-X-ray optics, and could greatly assist the realization of fully coherent X-ray sources, such as X-ray free-electron laser oscillators [1][2][3] . Diamond is a material with superlative physical qualities: high mechanical hardness, high thermal conductivity, high dispersion index, high radiation hardness, high hole and electron mobilities, low thermal expansion and chemically inert 4 . Technological applications of diamond crystals are increasing not only in the traditional fields of cutting, grinding and polishing tools, but also in high-tech applications, such as diamond-based electronic devices, wide-bandgap radiation detectors, ultraviolet-emitting diodes, biochemical sensors, high-pressure cells and thermal sinks, to name only a few. Very recently, diamond crystals have been identified as indispensable for the realization of X-ray free-electron laser oscillators (XFELOs), next-generation hard-X-ray sources of the highest average and peak brightness and extremely narrow bandwidth 1,2 . The special role of diamonds in the feasibility of the XFELOs is due to their outstanding reflectivity for hard X-rays in Bragg diffraction, thus far only predicted in theory (Fig. 1a).The high reflectivity of crystals in Bragg diffraction is intimately connected with the perfect crystal structure. Progress in fabrication, characterization and X-ray optics applications of synthetic diamonds was substantial in the past decade [5][6][7][8][9][10][11][12][13] . Still the diamond crystals available commercially as a rule suffer from defects: dislocations, stacking faults, inclusions, impurities and so on. Synthetic high-purity (type IIa, low nitrogen content) crystals grown with a high-pressure, high-temperature technique are generally considered to have the highest crystal quality and the lowest density of defects among commercially available diamonds 10,13 . X-ray topography studies have demonstrated crystals with relatively large 4×4 mm 2 defect-free areas 13 . However, critical outstanding questions remain o...
Obtaining a burning plasma is a critical step towards self-sustaining fusion energy1. A burning plasma is one in which the fusion reactions themselves are the primary source of heating in the plasma, which is necessary to sustain and propagate the burn, enabling high energy gain. After decades of fusion research, here we achieve a burning-plasma state in the laboratory. These experiments were conducted at the US National Ignition Facility, a laser facility delivering up to 1.9 megajoules of energy in pulses with peak powers up to 500 terawatts. We use the lasers to generate X-rays in a radiation cavity to indirectly drive a fuel-containing capsule via the X-ray ablation pressure, which results in the implosion process compressing and heating the fuel via mechanical work. The burning-plasma state was created using a strategy to increase the spatial scale of the capsule2,3 through two different implosion concepts4–7. These experiments show fusion self-heating in excess of the mechanical work injected into the implosions, satisfying several burning-plasma metrics3,8. Additionally, we describe a subset of experiments that appear to have crossed the static self-heating boundary, where fusion heating surpasses the energy losses from radiation and conduction. These results provide an opportunity to study α-particle-dominated plasmas and burning-plasma physics in the laboratory.
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