High temperature cuprate superconductors consist of stacked CuO2 planes, with primarily two dimensional electronic band structures and magnetic excitations [1,2], while superconducting coherence is three dimensional. This dichotomy highlights the importance of out-of-plane charge dynamics, believed to be incoherent in the normal state [3,4], yet lacking a comprehensive characterization in energy-momentum space. Here, we use resonant inelastic x-ray scattering (RIXS) with polarization analysis to uncover the pure charge character of a recently discovered collective mode in electron-doped cuprates [5-7]. This mode disperses along both the in-and, importantly, out-of-plane directions, revealing its three dimensional nature. The periodicity of the out-of-plane dispersion corresponds to the CuO2 plane distance rather than the crystallographic c-axis lattice constant, suggesting that the interplane Coulomb interaction drives the coherent out-of-plane charge dynamics. The observed properties are hallmarks of the long-sought acoustic plasmon, predicted for layered systems [8-13] and argued to play a substantial role in mediating high temperature superconductivity [13-15]. The charge dynamics of systems with periodically stacked quasi-two dimensional (2D) conducting planes are drastically affected in the presence of poorly screened interplane Coulomb interactions. In a simple layered electron gas model with conducting planes separated by dielectric spacers [8-10], the dispersion of plasmons, the collective electronic modes of the charge dynamics, evolves from optical-like to acoustic-like as a function of out-of-plane momentum qz [Fig. 1(a)], a behavior distinct from that in either pure 2D or isotropic 3D systems.For superconducting cuprates, similar charge dynamics have been postulated since they consist of conducting CuO2 planes stacked along the c-axis with poor out-of-plane screening [11][12][13]. While plasmons were observed in various spectroscopic studies at the Brillouin zone center [4,16,17] and by transmission electron energy loss spectroscopy (EELS) typically exploring in-plane
An understanding of the high-temperature copper oxide (cuprate) superconductors has eluded the physics community for over thirty years and represents one of the greatest unsolved problems in condensed matter physics. Particularly enigmatic is the normal state from which superconductivity emerges, so much so that this phase has been dubbed a “strange metal.” In this article, we review recent research into this strange metallic state as realized in the electron-doped cuprates with a focus on their transport properties. The electron-doped compounds differ in several ways from their more thoroughly studied hole-doped counterparts, and understanding these asymmetries of the phase diagram may prove crucial to developing a final theory of the cuprates. Most of the experimental results discussed in this review have yet to be explained and remain an outstanding challenge for theory.
The two-dimensional electron gas in SrTiO3 created by an overlayer of amorphous LaAlO3 is compared with those at the TiO2-terminated surfaces of rutile and anatase. Differences in conductivity are explained in terms of the limiting Ti-O-Ti bond angles (orbital corrugation), band dispersion, and polaron formation. At 300 K, the sheet conductivity and mobility of anatase exceed those for SrTiO3 or rutile by one or two orders of magnitude, respectively. The electrons in rutile become localized below 25 K.
We report ab-plane Hall Effect and magnetoresistivity measurements on La 2-x Ce x CuO 4 thin films as a function of doping for magnetic fields up to 14T and temperatures down to 1.8K. A dramatic change in the low temperature (1.8 K) normal state Hall coefficient is found near a doping Ce=0.14. This, along with a nonlinear Hall resistance as a function of magnetic field, suggests that the Fermi surface reconstructs at a critical doping of Ce= 0.14. A competing antiferromagnetic phase is the likely cause of this Fermi surface reconstruction. Low temperature linear-in-T resistivity is found at Ce=0.14, but anomalously, also at higher doping. We compare our data with similar behavior found in hole-doped cuprates at a doping where the pseudogap ends.
The confinement of the two-dimensional electron gas (2DEG), preferential occupancy of the Ti 3d orbital, and strong spin-orbit coupling at the LaAlO 3 /SrTiO 3 interface play a significant role in its emerging properties. Here we report a fourfold oscillation in the anisotropic magnetoresistance (AMR) and planar Hall effect (PHE) at the LaAlO 3 /SrTiO 3 heterointerface. We evaluate the carrier confinement effects on the AMR and find that the fourfold oscillation appears only for the case of 2DEG systems while it is twofold for the three-dimensional system. The AMR behavior is further found to be sensitive to applied electric field, emphasizing the significance of spin-orbit coupling at the interface. These confinement effects suggest that the magnetic interactions are predominant at the interface, and the gate electric field modulation of AMR shows the tunability of magnetic interactions. As the fourfold oscillation fits well to the phenomenological model for a cubic symmetry system, this suggests that the origin of the oscillation may be linked to the anisotropy in magnetic scattering arising from the interaction of electrons with the localized magnetic moments coupled to the crystal symmetry. The observed large PHE further indicates the in-plane nature of magnetic ordering that arises from the in-plane Ti 3d xy orbitals.
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.
customersupport@researchsolutions.com
10624 S. Eastern Ave., Ste. A-614
Henderson, NV 89052, USA
This site is protected by reCAPTCHA and the Google Privacy Policy and Terms of Service apply.
Copyright © 2024 scite LLC. All rights reserved.
Made with 💙 for researchers
Part of the Research Solutions Family.