Self-assembly is one of the most promising strategies for making functional materials at the nanoscale, yet new design principles for making self-limiting architectures, rather than spatially unlimited periodic lattice structures, are needed. To address this challenge, we explore the trade-offs between addressable assembly and self-closing assembly of a specific class of self-limiting structures: cylindrical tubules. We make triangular subunits using DNA origami that have specific, valencelimited interactions and designed binding angles, and study their assembly into tubules that have a self-limited width that is much larger than the size of an individual subunit. In the simplest case, the tubules are assembled from a single component by geometrically programming the dihedral angles between neighboring subunits. We show that the tubules can reach many micrometers in length and that their average width can be prescribed through the dihedral angles. We find that there is a distribution in the width and the chirality of the tubules, which we rationalize by developing a model that considers the finite bending rigidity of the assembled structure as well as the mechanism of self-closure. Finally, we demonstrate that the distributions of tubules can be further sculpted by increasing the number of subunit species, thereby increasing the assembly complexity, and demonstrate that using two subunit species successfully reduces the number of available end states by half. These results help to shed light on the roles of assembly complexity and geometry in self-limited assembly and could be extended to other self-limiting architectures, such as shells, toroids, or triply-periodic frameworks.

Viscous fingering patterns can form at the interface between two immiscible fluids confined in the gap between a pair of flat plates; whenever the fluid with lower viscosity displaces the one of higher viscosity the interface is unstable. For miscible fluids the situation is more complicated due to the formation of interfacial structure in the thin dimension spanning the gap. Here we study the effect of the inherent diffusion between the two miscible fluids on this structure and on the viscous fingering patterns that emerge. We discover an unexpected transition separating two distinct regimes where the pattern morphologies and mode of onset are different. This transition is marked by a regime of transient stability as the structure of the fingers evolves from having three-dimensional structure to being quasi-two dimensional. The presence of diffusion allows an instability to form where it was otherwise forbidden. arXiv:1803.07597v2 [physics.flu-dyn]

Cerenkov technology is often the optimal choice for particle identification in high energy particle collision applications. Typically, the most challenging regime is at high pseudorapidity (forward) where particle identification must perform well at high high laboratory momenta. For the upcoming Electron Ion Collider (EIC), the physics goals require hadron ($\pi$, K, p) identification up to $\sim$~50 GeV/c. In this region Cerenkov Ring-Imaging is the most viable solution.\newline The speed of light in a radiator medium is inversely proportional to the refractive index. Hence, for PID reaching out to high momenta a small index of refraction is required. Unfortunately, the lowest indices of refraction also result in the lowest light yield ($\frac{dN_\gamma}{dx} \propto \sin^2{\left(\theta_C \right)}$) driving up the radiator length and thereby the overall detector cost. In this paper we report on a successful test of a compact RICH detector (1 meter radiator) capable of delivering in excess of 10 photoelectrons per ring with a low index radiator gas ($CF_4$). The detector concept is a natural extension of the PHENIX HBD detector achieved by adding focusing capability at low wavelength and adequate gain for high efficiency detection of single-electron induced avalanches. Our results indicate that this technology is indeed a viable choice in the forward direction of the EIC. The setup and results are described within.Comment: 10 pages, 15 figure

Self-assembly is one of the most promising strategies for making functional materials at the nanoscale, yet new design principles for making self-limiting architectures, rather than spatially unlimited periodic lattice structures, are needed. To address this challenge, we explore the tradeoffs between addressable assembly and self-closing assembly of a specific class of self-limiting structures: cylindrical tubules. We make triangular subunits using DNA origami that have specific, valence-limited interactions and designed binding angles, and we study their assembly into tubules that have a self-limited width that is much larger than the size of an individual subunit. In the simplest case, the tubules are assembled from a single component by geometrically programming the dihedral angles between neighboring subunits. We show that the tubules can reach many micrometers in length and that their average width can be prescribed through the dihedral angles. We find that there is a distribution in the width and the chirality of the tubules, which we rationalize by developing a model that considers the finite bending rigidity of the assembled structure as well as the mechanism of self-closure. Finally, we demonstrate that the distributions of tubules can be further sculpted by increasing the number of subunit species, thereby increasing the assembly complexity, and demonstrate that using two subunit species successfully reduces the number of available end states by half. These results help to shed light on the roles of assembly complexity and geometry in self-limited assembly and could be extended to other self-limiting architectures, such as shells, toroids, or triply periodic frameworks.