Biodegradable and biocompatible elastic materials for soft robotics, tissue engineering or stretchable electronics with good mechanical properties, tunability, modifiability, or healing properties drive technological advance, yet they are not durable under ambient conditions nor combine all attributes in a single platform. We have developed a versatile gelatin-based biogel, which is highly resilient with outstanding elastic characteristics yet degrades fully when disposed. It self-adheres, is rapidly healable and derived entirely from natural and food-safe constituents. We merge for the first time all favorable attributes in one material that is easy to reproduce, scalable and low-cost in production under ambient conditions. This biogel is a step towards durable, lifelike soft robotic and electronic systems that are sustainable and closely mimic their natural antetypes. Main: In 2025, an estimated 6 million tons of garbage will be generated per day 1 , with tech disposables being a rapidly growing contributor. End-of-lifetime appliances contain valuable materials that are laborious in recovery or toxic substances that are readily released into nature through landfilling or improper treatment 2. Biodegradable 3-6 and transient systems 7 are promising routes towards closing the loop on waste generation and create new opportunities for secure systems, but often at the cost of compromises in performance. Complex biological systems bridge this gap. They unite seemingly antagonistic properties-tough yet adaptive, durable and self-healing yet degradable-allowing them to perform a myriad of intricate tasks. Embodiments of technologies that intimately interface with humans naturally benefit from mimicking such soft, functional forms. A range of biomimetic systems 8 including soft machines 9 and electronic skins 10 achieve a high level of functionality by introducing self-healing 11,12 , intrinsic stretchability 13 , or the insightful merging of soft-to-hard materials 14. Waste flow issues and in vivo applications that avoid multiple surgeries are tackled with inextensible devices in the form of edible 3,15 and transient electronics 7,16. However, introducing stretchability to degradable devices remains challenging. Recent approaches focusing on stretchable biodegradable sensors 5 require expensive materials and are still wired to bulky measurement systems hindering implementation as wearable devices. Challenges here stem from the diverse material requirements,
Rigid electromagnetic actuators serve our society in a myriad of ways for more than 200 years. However, their bulky nature restricts close collaboration with humans. Here, we introduce soft electromagnetic actuators (SEMAs) by replacing solid metal coils with liquid-metal channels embedded in elastomeric shells. We demonstrate human-friendly, simple, stretchable, fast, durable, and programmable centimeter-scale SEMAs that drive a soft shark, interact with everyday objects, or rapidly mix a dye with water. A multicoil flower SEMA with individually controlled petals blooms or closes within tens of milliseconds, and a cubic SEMA performs programmed, arbitrary motion sequences. We develop a numerical model supporting design and opening potential routes toward miniaturization, reduction of power consumption, and increase in mechanical efficiency. SEMAs are electrically controlled shape-morphing systems that are potentially empowering future applications from soft grippers to minimally invasive medicine.
High-speed locomotion is an essential survival strategy for animals, allowing populating harsh and unpredictable environments. Bio-inspired soft robots equally benefit from versatile and ultrafast motion but require appropriate driving mechanisms and device designs. Here, we present a class of small-scale soft electromagnetic robots made of curved elastomeric bilayers, driven by Lorentz forces acting on embedded printed liquid metal channels carrying alternating currents with driving voltages of several volts in a static magnetic field. Their dynamic resonant performance is investigated experimentally and theoretically. These robust and versatile robots can walk, run, swim, jump, steer and transport cargo. Their tethered versions reach ultra-high running speeds of 70 BL/s (body lengths per second) on 3D-corrugated substrates and 35 BL/s on arbitrary planar substrates while their maximum swimming speed is 4.8 BL/s in water. Moreover, prototype untethered versions run and swim at a maximum speed of 2.1 BL/s and 1.8 BL/s, respectively.
The hygroscopic nature of cellulose-based materials poses a challenge in utilising paper for printed electronics. Adsorbed moisture strongly modulates the conductive and dielectric properties of paper. While affecting the function of printed electronic elements, this behaviour is beneficial for low-cost humidity sensing. Here we describe a simple, sensitive paper-based sensor with a pair of inkjet-printed interdigitated electrodes for analysing water sorption of cellulose over a wide range of relative humidity from 10% to 90%. Impedance spectroscopy between 100 Hz and 1 MHz reveals the humidity-dependent electrical properties of paper. We show in particular that measurements at 1 MHz provide reliable information about the water adsorption and desorption of paper. In contrast, testing at frequencies below 200 kHz is dominated by ionic electrode polarisation, masking the water sorption kinetics of the sensor. Transient adsorption follows nearly an exponential function, while desorption is described by a stretched exponential law. At equilibrated conditions, the effective paper permittivity measured during adsorption and desorption is characterised by a Guggenheim-Anderson-de Boer sorption isotherm which allows for a quantitative evaluation of the sorption hysteresis. Our means of sensing provides a simple and practical method of recording and analysing simultaneously conductivity and permittivity as well as wetting and drying of moist paper.
Embedded sensors are key to optimizing processes and products; they collect data that allow time, energy, and materials to be saved, thereby reducing costs. After production, they remain in place and are used to monitor the long‐term structural health of buildings or aircraft. Fueled by climate change, sustainable construction materials such as wood and fiber composites are gaining importance. Current sensors are not optimized for use with these materials and often act as defects that cause catastrophic failures. Here, flexible, highly permeable, and imperceptible sensors (iSens) are introduced that integrate seamlessly into a component. Their porous substrates are readily infused with adhesives and withstand harsh conditions. In situ resistive temperature measurements and capacitive sensing allows monitoring of adhesives curing as used in wooden structures and fiber composites. The devices also act as heating elements to reduce the hardening time of the glue. Results are analyzed using numerical simulations and theoretical analysis. The suggested iSens technology is widely applicable and represents a step towards realizing the Internet of Things for construction materials.
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