Although some progress has been made on stretchable supercapacitors, traditional stretchable supercapacitors fabricated by predesigning structured electrodes for device assembling still lack the device-level editability and programmability. To adapt to wearable electronics with arbitrary configurations, it is highly desirable to develop editable supercapacitors that can be directly transferred into desirable shapes and stretchability. In this work, editable supercapacitors for customizable shapes and stretchability using electrodes based on mechanically strengthened ultralong MnO nanowire composites are developed. A supercapacitor edited with honeycomb-like structure shows a specific capacitance of 227.2 mF cm and can be stretched up to 500% without degradation of electrochemical performance, which is superior to most of the state-of-the-art stretchable supercapacitors. In addition, it maintains nearly 98% of the initial capacitance after 10 000 stretch-and-release cycles under 400% tensile strain. As a representative of concept for system integration, the editable supercapacitors are integrated with a strain sensor, and the system exhibits a stable sensing performance even under arm swing. Being highly stretchable, easily programmable, as well as connectable in series and parallel, an editable supercapacitor with customizable stretchability is promising to produce stylish energy storage devices to power various portable, stretchable, and wearable devices.
Articles you may be interested inEffect of nanocrystallization on the structure and the magnetic properties of Nd-Fe-Co-Al-B glassy alloy
Influence of ribbon thickness on the formation and magnetic properties of melt-spun Fe-Co-Nd-Dy-B metallic glassesThe glass-forming ability, thermal stability, and magnetic properties have been investigated for an Fe 67 Co 9.4 Nd 3.1 Dy 0.5 B 20 glassy alloy with a large supercooled liquid of 48 K before crystallization prepared by copper mold casting. The glassy phase is formed in a rod form with a diameter of 0.5 mm. The crystallized nanocomposite structure consists of Fe 3 B, ␣-Fe, and Nd 2 Fe 14 B phases, and the remanence (B r ), coercivity ( i H c ) and maximum energy product (BH) max are 1.19 T, 244 kA/m, and 92.7 kJ/m 3 , respectively, for the rod of 0.5 mm in diameter annealed at 913 K for 600 s.
Platinum
telluride (PtTe2) has garnered significant
research enthusiasm owing to its unique characteristics. However,
large-scale synthesis of PtTe2 toward potential photoelectric
and photovoltaic application has not been explored yet. Herein, we
report direct tellurization of Pt nanofilms to synthesize large-area
PtTe2 films and the influence of growth conditions on the
morphology of PtTe2. Electrical analysis reveals that the
as-grown PtTe2 films exhibit typical semimetallic behavior,
which is in agreement with the results of first-principles density
functional theory (DFT) simulation. Moreover, the combination of multilayered
PtTe2 and Si results in the formation of a PtTe2/Si heterojunction, exhibiting an obvious rectifying effect. Moreover,
the PtTe2-based photodetector displays a broadband photoresponse
to incident radiation in the range of 200–1650 nm, with the
maximum photoresponse at a wavelength of ∼980 nm. The R and D* of the PtTe2-based
photodetector are found to be 0.406 A W–1 and 3.62
× 1012 Jones, respectively. In addition, the external
quantum efficiency is as high as 32.1%. On the other hand, the response
time of τrise and τfall is estimated
to be 7.51 and 36.7 μs, respectively. Finally, an image sensor
composed of a 8 × 8 PtTe2-based photodetector array
was fabricated, which can record five near-infrared (NIR) images under
980 nm with a satisfying resolution. The result demonstrates that
the as-prepared PtTe2 material will be useful for application
in NIR optoelectronics.
Organic–inorganic halide perovskite solar cells (PSCs) have shown a significant growth in power conversion efficiencies (PCEs) during last decade. Progress in device architecture and high‐quality perovskite film fabrication has led to an incredible efficiency over 25% in close to a decade. Developments in solution‐based thin film deposition techniques for perovskite layer preparation in PSCs provide low cost and ease of process for their manufacturing, making them a potential contender in future solar energy harvesting technologies. From small area single solar cells to large area perovskite solar modules, solvents play crucial roles in thin film quality and therefore, the device performance and stability. A comprehensive overview of solvent engineering toward achieving the highest qualities for perovskite light absorbing layers with various compositions and based on different fabrication processes is provided in this review. The mechanisms indicating the essential roles a solvent, or a solvent mixture can play to improve the crystallinity, uniformity, coverage and surface roughness of the perovskite films, are discussed. Finally, the role of solvent engineering in transferring from small area laboratory scale PSC fabrication to large area perovskite film deposition processes is explored.
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