Recently released hourly particular matter (PM:PM2.5 and PM10) and gaseous pollutants (SO2, NO2, CO, and O3) data observed in Qingdao, Hangzhou, and Xiamen from 2015 to 2019 were utilized to reveal the current situation of air pollution over eastern coastal China. The PM pollution situation over the three metropolises ameliorated during studied period with the concentrations decreasing about 20–30%. Gas pollutants, excepting SO2, generally exhibit no evident reduction tendencies, and a more rigorous control standard on gaseous pollutants is neededEven for the year 2018 with low pollution levels among the study period, these levels (<10% of PM2.5, <6% of PM10, and <15% of O3) surpass the Grade II of the Chinese Ambient Air Quality Standard (CAAQS) over these metropolises of eastern coast China. No matter in which year, both SO2 and CO concentrations are always below the Grade-II standards. According to the comparative analysis of PM2.5/PM10 and PM2.5/CO during episode days and non-episode days, the formation of secondary aerosols associated with stagnant weather systems play an important role in the pollutant accumulation as haze episodes occurred. The stronger seasonal variations and higher magnitude occur in Qingdao and Hangzhou, while weaker seasonal variations and lower magnitudes occur in Xiamen. In Qingdao and Hangzhou, PM, NO2, SO2, and CO show relatively high levels in the cold wintertime and low levels in summer, whereas O3 shows a completely opposite pattern. Xiamen exhibits high levels of all air pollutants except O3 in spring due to its subtropical marine monsoon climate with mild winters. According to the back trajectory hierarchical clustering and concentration weighted trajectory (CWT) analysis, the regional transmission from adjacent cities has a significant impact on the atmospheric pollutant concentrations under the control of the prejudiced winds. Thus, besides local emission reduction, strengthening regional environmental cooperation and implementing joint prevention are effective measures to mitigate air pollution in the eastern coastal areas of China.

The wet deposition flux of black carbon (BC) over the Sichuan Basin is studied on the basis of the MERRA-2 data from 1981 to 2020, aiming at investigating high BC wet deposition flux in China in terms of long-term spatial-temporal trends and influences of BC column mass density and precipitation. In China, the largest BC wet deposition flux with a regionally-averaged value of 1.00 × 10−2 μg m−2 s−1 over the Sichuan Basin is observed, especially in the western and southern regions of the Basin with values as high as 2.20 × 10−2 μg m−2 s−1. The seasonality of BC wet deposition flux over the Sichuan Basin depicts maximum levels in autumn, moderate levels in spring and winter, and minimum levels in summer. The monthly mean BC wet deposition flux varies almost twofold, ranging from the lowest average value of 8.05 × 10−3 μg m−2 s−1 in July to the highest 1.28 × 10−2 μg m−2 s−1 in October. This study suggests that BC column mass density and precipitation are two significant factors affecting high BC wet deposition flux, whereas BC wet deposition flux is more related to BC column mass density than to precipitation over the Sichuan Basin.