Anisotropic particles have been widely used to make micro/nanomotors that convert chemical, ultrasonic, electrical, or magnetic energy into mechanical energy. The moving directions of most colloidal motors are, however, difficult to control. For example, asymmetric dimers with two lobes of different sizes, ζ-potential, or chemical composition have shown rich propulsion behaviors under alternating current (AC) electric fields due to unbalanced electrohydrodynamic flow. While they always propel in a direction perpendicular to the applied electric field, their moving directions along the substrate are hard to control, limiting their applications for cargo delivery. Inspired by two separate engine and steering wheel systems in automobiles, we use orthogonally applied AC electric field and direct current (DC) magnetic field to control the dimer's speed and direction independently. To this end, we first synthesize magnetic dimers by coating dopamine-functionalized nanoparticles on geometrically asymmetric polystyrene dimers. We further characterize their static and dynamic susceptibilities by measuring the hysteresis diagram and rotation speed experimentally and comparing them with theoretical predictions. The synthesized dimers align their long axes quickly with a planar DC magnetic field, allowing us to control the particles' orientation accurately. The propulsion speed of the dimers, on the other hand, is tunable by an AC electric field applied perpendicularly to the substrate. As a result, we can direct the particle's motion with predesigned trajectories of complex shapes. Our bulk-synthesis approach has the potential to make other types of magnetically anisotropic particles. And the combination of electric and magnetic fields will help pave the way for the assembly of magnetically anisotropic particles into complex structures.

The remarkable efficiency and dynamics of micromachines in living organisms have inspired researchers to make artificial microrobots for targeted drug delivery, chemical sensing, cargo transport, and waste remediation applications. While several self- and directed-propulsion mechanisms have been discovered, the phoretic force has to be generated via either asymmetric surface functionalization or sophisticated geometric design of microrobots. As a result, many symmetric structures assembled from isotropic colloids are ruled out as viable microrobot possibilities. Here, we propose to utilize orientation control to actuate axially symmetric micro-objects with homogeneous surface properties, such as linear chains assembled from superparamagnetic microspheres. We demonstrate that the fore-and-aft symmetry of a horizontal chain can be broken by tilting it with an angle relative to the substrate under a two-dimensional magnetic field. A superimposed alternating current electric field propels the tilted chains. Our experiments and numerical simulation confirm that the electrohydrodynamic flow along the electrode is unbalanced surrounding the tilted chain, generating hydrodynamic stresses that both propel the chain and reorient it slightly toward the substrate. Our work takes advantage of external fields, where the magnetic field, as a driving wheel and brake, controls chain orientation and direction, while the electric field, as an engine, provides power for locomotion. Without the need to create complex-shaped micromotors with intricate building blocks, our work reveals a propulsion mechanism that breaks the symmetry of hydrodynamic flow by manipulating the orientation of a microscopic object.