Abstract. In January 2013, February 2014, December 2015 and December 2016
to 10 January 2017, 12 persistent heavy aerosol pollution episodes
(HPEs) occurred in Beijing, which received special attention from the public. During the HPEs, the precise
cause of PM2.5 explosive growth (mass concentration at least doubled in
several hours to 10 h) is uncertain. Here, we analyzed and estimated relative
contributions of boundary-layer meteorological factors to such growth, using
ground and vertical meteorological data. Beijing HPEs are generally
characterized by the transport stage (TS), whose aerosol pollution formation
is primarily caused by pollutants transported from the south of Beijing, and
the cumulative stage (CS), in which the cumulative explosive growth of
PM2.5 mass is dominated by stable atmospheric stratification
characteristics of southerly slight or calm winds, near-ground anomalous
inversion, and moisture accumulation. During the CSs, observed southerly weak
winds facilitate local pollutant accumulation by minimizing horizontal
pollutant diffusion. Established by TSs, elevated PM2.5 levels scatter
more solar radiation back to space to reduce near-ground temperature,
which very likely causes anomalous inversion. This surface cooling by
PM2.5 decreases near-ground saturation vapor pressure and increases
relative humidity significantly; the inversion subsequently reduces vertical
turbulent diffusion and boundary-layer height to trap pollutants and
accumulate water vapor. Appreciable near-ground moisture accumulation
(relative humidity> 80 %) would further enhance aerosol hygroscopic growth and
accelerate liquid-phase and heterogeneous reactions, in which incompletely
quantified chemical mechanisms need more investigation. The positive
meteorological feedback noted on PM2.5 mass explains over 70 % of cumulative
explosive growth.
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