Direct conversion of biomass to carbon aerogel provides a promising approach to developing absorbent materials for spilled oils and organic solvents recovery. In this work, three-dimensional carbon aerogels were fabricated via a hydrothermal and post-pyrolysis process using winter melon as the only raw materials. The winter melon carbon aerogel (WCA) prepared shows a low density of 0.048 g/cm 3 , excellent hydrophobicity with a water contact angle of 135°, and selective absorption for organic solvents and oils. The absorption capacity of WCA for organic solvents and oils can be 16−50 times its own weight. Moreover, distillation can be employed to recover WCA and harvest the pollutants. Over five absorption−harvesting cycles, the absorption capacity of WCA to organic solvents and low boiling point oils can recover almost 100% of its starting capacity. With a combination of low-cost biomass as raw materials, green preparation process, low density, and excellent hydrophobicity, WCA as an absorber has great potential in application of spilled oil recovery and environmental protection.
Freestanding, mechanically stable, and highly electrically conductive graphene foam (GF) is formed with a two-step facile, adaptable, and scalable technique. This work also demonstrates the formation of graphene foam with tunable densities and its use as strain/pressure sensor for both high and low strains and pressures.
We introduce a simple method to fabricate a highly flexible resistive-type strain sensor composed of carbon paper (CP) and polydimethylsiloxane (PDMS) elastomer. The key resistance sensitive material of the sensor, carbon paper, is prepared from tissue paper by a simple high-temperature pyrolysis process. At the same time, the as-fabricated CP/PDMS strain senor is highly sensitive to applied strain with a gauge factor (GF) of 25.3, almost 10 times higher than that of conventional metallic strain gauge. Furthermore, the response of CP/PDMS strain sensor under cyclic tensile strain with a peak strain of 3% was also investigated, which exhibits fast and steady response with excellent durability within the frequency range of 0.01-10Hz. Finally, we demonstrate the successful utilization of the CP/PDMS strain sensor as wearable electronics in breath monitoring and robot controlling. The eminent performance, low material cost, and facile fabrication process make the CP/PDMS strain sensor exceptionally promising in flexible, stretchable and wearable electronics.
Solution-processed semiconducting transition metal dichalcogenides (TMDs) are at the centre of an ever-increasing research effort in printed (opto)electronics. However, device performance is limited by structural defects resulting from the exfoliation process and poor inter-flake electronic connectivity.Here, we report a new molecular strategy to boost the electrical performance of TMD-based devices via the use of dithiolated conjugated molecules, to simultaneously heal sulfur vacancies in solutionprocessed transition metal disulfides (MS2) and covalently bridge adjacent flakes, thereby promoting percolation pathways for the charge transport. We achieve a reproducible increase by one order-ofmagnitude in field-effect mobility (µFE), current ratios (ION / IOFF), and switching times (τS) of liquid-gated transistors, reaching 10 -2 cm 2 V -1 s -1 , 10 4 , and 18 ms, respectively. Our functionalization strategy is an universal route to simultaneously enhance the electronic connectivity in MS2 networks and tailor on demand their physicochemical properties according to the envisioned applications.
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