A focusing optics that can provide a sub-micrometre high-flux probe for soft X-ray micrometre-scale angle-resolved photoemission spectroscopy (ARPES) is proposed. A monolithic Wolter-type mirror with a large acceptance, achromatism and small comatic aberration was designed and evaluated. A focused beam size of 0.4 µm (vertical) × 4 µm (horizontal), a high throughput of 59% and a high tolerance of 1.6 mrad to the pitching error were realized at a photon energy of 1000 eV. A Wolter-type mirror can be practically employed as a stable sub-micrometre focusing mirror with high throughput in ARPES applications.

In X-ray focusing, grazing incidence mirrors offer advantages of no chromatic aberration and high focusing efficiency. Although nanofocusing mirrors have been developed for the hard X-ray region, there is no mirror with nanofocusing performance in the soft X-ray region. Designing a system with the ability to focus to a beam size smaller than 100 nm at an X-ray energy of less than 1 keV requires a numerical aperture larger than 0.01. This leads to difficulties in the fabrication of a soft X-ray focusing mirror with high accuracy. Ellipsoidal mirrors enable soft X-ray focusing with a high numerical aperture. In this study, we report a production process for ellipsoidal mirrors involving mandrel fabrication and replication processes. The fabricated ellipsoidal mirror was assessed under partial illumination conditions at the soft X-ray beamline (BL25SU) of SPring-8. A focal spot size of less than 250 nm was confirmed at 300 eV. The focusing tests indicated that the proposed fabrication process is promising for X-ray mirrors that have the form of a solid of revolution, including Wolter mirrors.

Ellipsoidal mirrors are promising optical devices for soft x-ray focusing. A fabrication process consisting of master fabrication and replication has been developed to produce ellipsoidal mirrors with wide apertures of approximately 10 mm. In the present study, the focusing performance of an ellipsoidal mirror was evaluated using soft x-rays in the soft x-ray beamline BL25SU-a of SPring-8. The focus sizes were measured at photon energies of 300, 400, and 500 eV. A quantitative figure error of the ellipsoidal mirror was also evaluated by analyzing the wavefield of the focused beam retrieved using ptychography. The figure error distributions measured at different photon energies agreed with each other at a root mean square level of 1 nm. The developed focusing system can be used for various types of microscopy, allowing the use of a wide range of x-ray energies.

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