The electrocatalytic splitting of water via hydrogen evolution reaction (HER) is one of the most efficient technologies for hydrogen production, while the massive consumption of precious Pt‐based catalysts hinders its commercialization, bringing an urgent task to explore low‐cost and earth‐abundant alternatives. Herein, a cost‐efficient system composed of metal Pt/molybdenum disulphide (MoS2) nanosheets hybrids for the HER by auxiliary of solar light is reported. The uniformly Pt nanoparticle decorated MoS2 sheets can be easily obtained under hydrothermal condition using oleylamine as capping agent and N,N‐dimethylmethanamide (DMF) as intercalation molecule for MoS2 exfoliation. The Pt/MoS2 hybrid shows a significantly enhanced HER activity compared with bare MoS2 due to enhancing conductivity and reducing overpotential by electron transport between Pt and MoS2. As a result, a Tafel slope of 38 mV per decade is obtained, suggesting a highly efficient Volmer–Heyrovsky reaction of hydrogen evolution.
Hf 1-x Ti x O 2 dense ceramics were prepared by a standard solid-state reaction process, and the microwave dielectric properties in a wide frequency range were determined together with structure evolution. With increasing x, the structure gradually changed from HfO 2 -based solid solution (monoclinic in space group P2 1 /c, x ≤ 0.05) to HfTiO 4 (orthorhombic in space group Pbcn, x = 0.5), and the two phase regions were determined for 0.1 ≤x < 0.5 and x = 0.55. The microwave dielectric properties of HfO 2 ceramics at 10 GHz were determined as ε r = 14, Qf = 24 500 GHz, τ f = -50 ppm/°C. With Ti-substitution, the microwave dielectric characteristics, especially the Qf value, could be significantly improved, and the best combination of microwave dielectric characteristics was achieved at x = 0.05: ε r = 17, Qf = 84 020 GHz (at 7.8 GHz) and 151 260 GHz (at 27.9 GHz), and τ f = -47 ppm/°C. The smallest temperature coefficient of resonance frequency (τ f = -4.8 ppm/°C) was obtained for x = 0.55 together with a Qf value of 52 370 GHz at 5.0 GHz and 60 390 GHz at 17.9 GHz, where the dielectric constant was 40. Moreover, Hf 1-x Ti x O 2 microwave dielectric ceramics might be very competitive in the future of mobile communication technology due to their excellent compatibility with Si.
A redundant lifting wavelet packet analysis based on variable parameter was presented, which was used to extract the weak fault features of bearing submerged in background noise. Through different choices of parameters in the design formula of predictor based on least square method of fitting, six asymmetric wavelets with various characteristics were constructed, which were then respectively used for redundant lifting wavelet packet decomposition to signal layer by layer. All the results obtained by decomposition were adopted to establish the objective function of minimum norm, through which the optimal wavelet that best matches the feature information is selected for each node signal. The node signals got by last decomposition were utilized for wavelet packet energy analysis, while the node signal with maximum energy was chosen for single branch reconstruction and envelop spectrum analysis. The proposed method above is applied to process the engineering data of bearing with fault and good results are gained by which the effectiveness of this method is well validated.
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