The
technological revolution of two-dimensional (2D) materials
provides vitality for ultrafast optics. Compared with other 2D materials,
indium sulfide (In2S3) has become an attractive
candidate material in the field of nonlinear optics because of its
high carrier mobility, ultrafast photoelectric sensitivity, medium
band gap, and high absorption coefficient. However, its nonlinear
optical effects have rarely been studied. In this work, we synthesized
2D β-In2S3 nanoplates using the hydrothermal
method. The saturable absorber based on β-In2S3 nanoplates has been investigated. The experimental results
demonstrated that the modulation depth and saturable intensity of
β-In2S3 are measured as 2.32% and 18.4
MW·cm–2, respectively, which indicates that
β-In2S3 has great potential in ultrafast
optics among emerging nonlinear optical materials. Using such unprecedented
properties, the mode-locked fiber laser with 247th (1.92 GHz) harmonic
mode locking is realized in the C-band for the first time to our knowledge.
This paves the way for exploring β-In2S3 as an outstanding nonlinear material for high-performance ultrafast
optics.