“…Recently, a burgeoning interest in three-terminal devices for artificial synapses has been observed, largely due to their nondestructive weight-update function, which benefits from the separation of writing (gate) and reading (drain) terminals. ,− The weight updates in these devices are governed by various charge-storage mechanisms, including interfacial traps, , floating gates, − ion intercalation, , and defects in dielectrics. , Additionally, three-terminal devices featuring charge-storage capabilities have been rigorously explored in the context of van der Waals heterostructures. These structures are composed of two-dimensional (2D) materials exhibiting distinct structural and material properties, − and have shown potential for nonvolatile electronic and optoelectronic memory applications. ,,− Notably, Large-scale MoS 2 floating-gate transistor arrays have been successfully fabricated, and the subsequent integration of these arrays into circuits has enabled the realization of logic-in-memory functionality, further highlighting the commercial prospects of three-terminal devices employing 2D materials. , However, these devices have not yet proven suitable for low-energy-consumption artificial synapse applications due to their limited operation speed. Although the floating gate configurationfeaturing uniform atomically sharp interfaces and a high gate coupling ratiocan address this issue, concerns regarding the complex fabrication processes remain. , As a result, it is crucial to meticulously design an alternative memory structure that can provide a viable solution to the low operation speed challenge.…”