With increasing the film area/layer, deteriorating in both smoothness and uniformity of thin-films frequently happen, which remains a barrier for making large-area quantum dot light-emitting diodes (QLEDs) by solution processes. Here, we demonstrated a facile all-solution process guided by the conical fiber array to write multi-layer ultrasmooth thin-films directly in centimeter scale. The side-by-side fibrous array helps to align surface tensions at the tri-phase contact line to facilitate large-area homogeneous deposition, which was verified by theoretical simulation. The Laplace pressure along individual conical fiber contributes to the steady liquid transfer. Thin-films with small roughness (< 2.03 nm) and large-area (2 2 cm 2) uniformity were prepared sequentially on the target substrate, leading to large-area highperformance QLEDs. The result offers new insights for fabricating large-area high-performance thin-film devices. Quantum dot light-emitting diodes (QLEDs) have attracted research attentions as the most promising nextgeneration display [1] and lighting [2] devices, because of the narrow spectral emission bandwidths, color tunability, and good photostability. [3] As a multi-layer thin-film device, sequential preparing functional layers on the target substrate were necessary, which have been normally realized by solution processes due to the mild conditions and easy operation. [4] For a high-performance QLED, high-quality thin-films with both small surface roughness and good uniformity are desirable for facilitating not only the charge transport within the film but the charge balance between neighboring layers. [5] So far, solution processes including spin coating, [6] inkjet printing, [7] and transfer printing [8] have been developed. However, these approaches suffered from the nonuniform deposition as the film area/layer increases, which remains a barrier for making large-area QLEDs. With increasing either the print area or the film layer, fluid