Abstract. The rapid response to the COVID-19 pandemic led to unprecedented decreases in
economic activities, thereby reducing the pollutant emissions. A random forest
(RF) model was applied to determine the respective contributions of
meteorology and anthropogenic emissions to the changes in air quality. The
result suggested that the strict lockdown measures significantly decreased primary
components such as Cr (−67 %) and Fe (−61 %) in
PM2.5 (p<0.01), whereas the higher relative humidity (RH) and
NH3 level and the lower air temperature (T) remarkably enhanced
the production of secondary aerosol, including SO42-
(29 %), NO3- (29 %), and NH4+
(21 %) (p<0.05). The positive matrix factorization (PMF) result
suggested that the contribution ratios of secondary formation (SF), industrial
process (IP), biomass burning (BB), coal combustion (CC), and road dust (RD)
changed from 36 %, 27 %, 21 %,
12 %, and 4 % before the COVID-19 outbreak to
44 %, 20 %, 20 %, 9 %, and
7 %, respectively. The rapid increase in the contribution ratio
derived from SF to PM2.5 implied that the intermittent haze events during
the COVID-19 period were characterized by secondary aerosol pollution, which was
mainly contributed by the unfavorable meteorological conditions and high
NH3 level.