The miniaturization and high frequency of future electromagnetic devices require soft magnetic composites with high permeability, high working frequency and low core loss. In this work, easy-plane amorphous FeSiBCr powders with a thickness of approximately 1~2 μm are obtained by planetary ball milling and successfully fabricated into an arranged soft magnetic composite by using a rotational magnetic field. The complex permeability spectrums of the composite are measured and analyzed. Due to the planar distribution of easy magnetization axes, the amorphous easy-plane FeSiBCr/Si-resin composite shows a permeability of 31 at 1MHz. The core loss of samples is measured from 100 KHz to 5 MHz and discussed in detail. The loss separated results illustrate the eddy current loss and excess loss can be effectively reduced in amorphous easy-plane FeSiBCr/Si-resin composite. These results indicate that, compared with the amorphous none easy-plane FeSiBCr/Si-resin composite, the permeability of the amorphous easy-plane FeSiBCr/Si-resin composite is effectively improved and the core loss is reduced, making it promising for the high-frequency application.