Elastomers that combined
excellent mechanical performance and healability are essential to
the advancement of stretchable electronics. However, the strength
and toughness of healable elastomers tend to be mutually exclusive.
Herein, a new strategy of the dynamic integrated moiety is developed
to construct covalent and noncovalent cross-linked polyurethane (CNPU)
elastomers. The covalent and noncovalent interactions synergistically
enhance the overall mechanical properties of polyurethane elastomers
such as tensile strength (48.8 MPa), toughness (282.9 MJ·m–3), stretchability (1740%), and healing efficiency
(116%). Finally, elastic conductive wires are fabricated with high
load capacity, stable electrical conductivity under static/dynamic
stretching, and robust healability to demonstrate the potential use
of CNPU elastomers in stretchable electronics.